Structure and reorientational dynamics of 1-F-adamantane

The polymorphism and the dynamics of a simple rigid molecule (1-fluoro-adamantane) have been studied by means of X-ray powder diffraction and broadband dielectric spectroscopy. At temperatures below the melting point, the molecule forms an orientationally disordered Phase I with a cubic-centered str...

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Detalles Bibliográficos
Autores: Ben Hassine, Bacem, Negrier, Philippe, Romanini, Michela|||0000-0002-1685-855X, Barrio Casado, María del|||0000-0003-3467-7581, Macovez, Roberto|||0000-0001-5026-9372, Kallel, A., Mondieig, Denise, Tamarit Mur, José Luis|||0000-0002-7965-0000
Tipo de recurso: artículo
Fecha de publicación:2016
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/89251
Acceso en línea:https://hdl.handle.net/2117/89251
https://dx.doi.org/10.1039/c6cp01144f
Access Level:acceso abierto
Palabra clave:Glass transition temperature
Adamantane
Supercooled liquids
Polymorphism (Crystallography)
Molecular dynamics
glass-transition
supercooled liquids
molecular motions
plasic phase
1-fluoroadamantane
relaxation
adamantane
crystals
polimorphism
temperature
Vidre -- Propietats físiques
Líquids -- Propietats tèrmiques
Polimorfisme
Dinàmica molecular
Àrees temàtiques de la UPC::Física::Física molecular
Àrees temàtiques de la UPC::Enginyeria química::Química física
Descripción
Sumario:The polymorphism and the dynamics of a simple rigid molecule (1-fluoro-adamantane) have been studied by means of X-ray powder diffraction and broadband dielectric spectroscopy. At temperatures below the melting point, the molecule forms an orientationally disordered Phase I with a cubic-centered structure (Phase I, Fm (3) over barm, Z = 4). This phase possesses eight equilibrium positions for the fluorine atom, with equal occupancy factors of 1/8. A solid-solid phase transition to a low-temperature tetragonal phase (Phase II, P (4) over bar2(1)c, Z = 2) reduces the statistical disorder to only four possible equivalent sites for the fluorine atom, with fractional occupancies of 1/4. The dynamics has been rationalized under the constraints imposed by the space group of the crystal structure determined by powder X-ray diffraction. The dielectric spectroscopy study reveals that the statistical disorder in Phase II is dynamic in character and is associated with reorientational jumps along the two-and three-fold axes. In the dielectric loss spectra, the cooperative (alpha) relaxation exhibits a shoulder on the high-frequency side. This remarkable finding clearly reveals the existence of two intrinsic reorientational processes associated with the exchange of the F atom along the four sites. In addition to such