Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films

The unparalleled loss-less electrical current conduction of high-temperature superconducting (HTS) materials encourages research on YBa2Cu3O7− (YBCO) to unravel opportunities toward numerous applications. Nonetheless, production costs and throughput of the commercialized HTS Coated Conductors (CCs)...

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Detalles Bibliográficos
Autores: Saltarelli, Lavinia, García, Diana, Soler Bru, Laia, Pach, Elzbieta, Gupta, Kapil, Sánchez Rodríguez, Daniel, Aguilar, Jordi, Fuentes, Víctor, Solano, Eduardo, Mocuta, Cristian, Farjas Silva, Jordi, Obradors, Xavier, Puig Molina, Teresa
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2025
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:10256/27388
Acceso en línea:http://hdl.handle.net/10256/27388
Access Level:acceso abierto
Palabra clave:Superconductors
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spelling Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ FilmsSaltarelli, LaviniaGarcía, DianaSoler Bru, LaiaPach, ElzbietaGupta, KapilSánchez Rodríguez, DanielAguilar, JordiFuentes, VíctorSolano, EduardoMocuta, CristianFarjas Silva, JordiObradors, XavierPuig Molina, TeresaSuperconductorsSuperconductorsThe unparalleled loss-less electrical current conduction of high-temperature superconducting (HTS) materials encourages research on YBa2Cu3O7− (YBCO) to unravel opportunities toward numerous applications. Nonetheless, production costs and throughput of the commercialized HTS Coated Conductors (CCs) are still limiting a worldwide spread. Transient liquid assisted growth (TLAG) is a non-equilibrium process displaying ultrafast growth rate which, when combined with chemical solution deposition (CSD), is emerging as a strong candidate to reduce the cost/performance ratio of YBCO superconductors. This study explores the influence of the (Ba:Cu) molar ratio of the transient liquid composition on the nucleation and growth mechanisms of TLAG. This enables an in-depth analysis of the critical role of the yttrium supersaturation in the transient liquids considering the out-of-equilibrium kinetic character of TLAG. Advanced characterization techniques, including in situ synchrotron X-ray diffraction, coupled to a multi-parameter analysis of the contributions to the physical performance, elucidate the influence of transient liquid supersaturation as driving force toward YBCO nucleation and growth. Understanding the fundamental role played by the initial ink composition allows to disentangle how to reach high superconducting performance. The fabrication of high-performance YBCO films through this novel, high-throughput growth methodology promotes the use of HTS materials in large scale power applicationsResearch funding: EU COST actions. Grant Numbers: CA20116, CA-21144; Spanish Ministry of Science and Innovation and the European Regional Development Fund. Grant Numbers: PID2021-127297OB-C21, FUNFUTURECEX2019-000917-S, Matrans42CEX2023-001263-S, PDC2022-133208-I00; Spanish Ministry of Science. Grant Numbers: PRE2019-090621, PRE2018-084537; Departament d'Innovació, Universitats i Empresa, Generalitat de Catalunya. Grant Number: BP00069; Direcció General de Recerca, Generalitat de Catalunya. Grant Number: 2021 SGR 00440; Fundación General CSIC. Grant Number: NGEU (Regulation (EU) 2020/2094); Ministerio de Ciencia e Innovación. Grant Numbers: PID2021-127297OB-C22, IJC2020-045520-I; HORIZON EUROPE European Research Council. Grant Numbers: ERC-2022-PoC-101081998, ERC-2019-PoC-8749 & HORIZON EUROPE European Innovation Council. Grant Number: ERC-2014-ADG-669504WileyAgencia Estatal de Investigación2025info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionpeer-reviewedapplication/pdfhttp://hdl.handle.net/10256/27388Advanced Materials, 2025, vol. undef, núm. undef, p. undefArticles publicats (D-F)Saltarelli, Lavinia García, Diana Soler Bru, Laia Pach, Elzbieta Gupta, Kapil Sánchez Rodríguez, Daniel&#8203 Aguilar, Jordi Fuentes, Víctor Solano, Eduardo Mocuta, Cristian Farjas Silva, Jordi Obradors, Xavier Puig Molina, Teresa 2025 Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films Advanced Materials undef undef undefreponame:Recercat. Dipósit de la Recerca de Catalunyainstname:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)Inglésinfo:eu-repo/semantics/altIdentifier/doi/10.1002/adma.202510660info:eu-repo/semantics/altIdentifier/issn/0935-9648info:eu-repo/semantics/altIdentifier/eissn/1521-4095PID2021-127297OB-C22info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-127297OB-C22Reconeixement 4.0 Internacionalhttp://creativecommons.org/licenses/by/4.0info:eu-repo/semantics/openAccessoai:recercat.cat:10256/273882026-05-29T05:05:01Z
dc.title.none.fl_str_mv Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films
title Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films
spellingShingle Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films
Saltarelli, Lavinia
Superconductors
Superconductors
title_short Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films
title_full Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films
title_fullStr Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films
title_full_unstemmed Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films
title_sort Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films
dc.creator.none.fl_str_mv Saltarelli, Lavinia
García, Diana
Soler Bru, Laia
Pach, Elzbieta
Gupta, Kapil
Sánchez Rodríguez, Daniel
Aguilar, Jordi
Fuentes, Víctor
Solano, Eduardo
Mocuta, Cristian
Farjas Silva, Jordi
Obradors, Xavier
Puig Molina, Teresa
author Saltarelli, Lavinia
author_facet Saltarelli, Lavinia
García, Diana
Soler Bru, Laia
Pach, Elzbieta
Gupta, Kapil
Sánchez Rodríguez, Daniel
Aguilar, Jordi
Fuentes, Víctor
Solano, Eduardo
Mocuta, Cristian
Farjas Silva, Jordi
Obradors, Xavier
Puig Molina, Teresa
author_role author
author2 García, Diana
Soler Bru, Laia
Pach, Elzbieta
Gupta, Kapil
Sánchez Rodríguez, Daniel
Aguilar, Jordi
Fuentes, Víctor
Solano, Eduardo
Mocuta, Cristian
Farjas Silva, Jordi
Obradors, Xavier
Puig Molina, Teresa
author2_role author
author
author
author
author
author
author
author
author
author
author
author
dc.contributor.none.fl_str_mv Agencia Estatal de Investigación
dc.subject.none.fl_str_mv Superconductors
Superconductors
topic Superconductors
Superconductors
description The unparalleled loss-less electrical current conduction of high-temperature superconducting (HTS) materials encourages research on YBa2Cu3O7− (YBCO) to unravel opportunities toward numerous applications. Nonetheless, production costs and throughput of the commercialized HTS Coated Conductors (CCs) are still limiting a worldwide spread. Transient liquid assisted growth (TLAG) is a non-equilibrium process displaying ultrafast growth rate which, when combined with chemical solution deposition (CSD), is emerging as a strong candidate to reduce the cost/performance ratio of YBCO superconductors. This study explores the influence of the (Ba:Cu) molar ratio of the transient liquid composition on the nucleation and growth mechanisms of TLAG. This enables an in-depth analysis of the critical role of the yttrium supersaturation in the transient liquids considering the out-of-equilibrium kinetic character of TLAG. Advanced characterization techniques, including in situ synchrotron X-ray diffraction, coupled to a multi-parameter analysis of the contributions to the physical performance, elucidate the influence of transient liquid supersaturation as driving force toward YBCO nucleation and growth. Understanding the fundamental role played by the initial ink composition allows to disentangle how to reach high superconducting performance. The fabrication of high-performance YBCO films through this novel, high-throughput growth methodology promotes the use of HTS materials in large scale power applications
publishDate 2025
dc.date.none.fl_str_mv 2025
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
peer-reviewed
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10256/27388
url http://hdl.handle.net/10256/27388
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.1002/adma.202510660
info:eu-repo/semantics/altIdentifier/issn/0935-9648
info:eu-repo/semantics/altIdentifier/eissn/1521-4095
PID2021-127297OB-C22
info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-127297OB-C22
dc.rights.none.fl_str_mv Reconeixement 4.0 Internacional
http://creativecommons.org/licenses/by/4.0
info:eu-repo/semantics/openAccess
rights_invalid_str_mv Reconeixement 4.0 Internacional
http://creativecommons.org/licenses/by/4.0
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.publisher.none.fl_str_mv Wiley
publisher.none.fl_str_mv Wiley
dc.source.none.fl_str_mv Advanced Materials, 2025, vol. undef, núm. undef, p. undef
Articles publicats (D-F)
Saltarelli, Lavinia García, Diana Soler Bru, Laia Pach, Elzbieta Gupta, Kapil Sánchez Rodríguez, Daniel&#8203 Aguilar, Jordi Fuentes, Víctor Solano, Eduardo Mocuta, Cristian Farjas Silva, Jordi Obradors, Xavier Puig Molina, Teresa 2025 Role of Liquid Composition in the Transient Liquid Assisted Growth of Superconducting YBa2Cu3O7-δ Films Advanced Materials undef undef undef
reponame:Recercat. Dipósit de la Recerca de Catalunya
instname:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
instname_str Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
reponame_str Recercat. Dipósit de la Recerca de Catalunya
collection Recercat. Dipósit de la Recerca de Catalunya
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15,81155

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