Strain-induced coupling of electrical polarization and structural defects in SrMnO3 films

Local perturbations in complex oxides, such as domain walls, strain and defects, are of interest because they can modify the conduction or the dielectric and magnetic response, and can even promote phase transitions. Here, we show that the interaction between different types of local perturbations i...

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Detalles Bibliográficos
Autores: Becher, Carsten, Maurel, Laura, Aschauer, Ulrich, Lilienblum, Martin, Magén, César, Meier, Dennis, Langenberg, Eric, Trassin, Morgan, Blasco, Javier, Krug, Ingo P., Algarabel, Pedro A., Spaldin, Nicola A., Pardo, José A., Fiebig, Manfred
Tipo de recurso: artículo
Estado:Versión enviada para evaluación y publicación
Fecha de publicación:2015
País:España
Institución:Universidad de Zaragoza
Repositorio:Zaguán. Repositorio Digital de la Universidad de Zaragoza
OAI Identifier:oai:zaguan.unizar.es:46954
Acceso en línea:http://zaguan.unizar.es/record/46954
Access Level:acceso abierto
Descripción
Sumario:Local perturbations in complex oxides, such as domain walls, strain and defects, are of interest because they can modify the conduction or the dielectric and magnetic response, and can even promote phase transitions. Here, we show that the interaction between different types of local perturbations in oxide thin films is an additional source of functionality. Taking SrMnO 3 as a model system, we use nonlinear optics to verify the theoretical prediction that strain induces a polar phase, and apply density functional theory to show that strain simultaneously increases the concentration of oxygen vacancies. These vacancies couple to the polar domain walls, where they establish an electrostatic barrier to electron migration. The result is a state with locally structured room-temperature conductivity consisting of conducting nanosized polar domains encased by insulating domain boundaries, which we resolve using scanning probe microscopy. Our 'nanocapacitor' domains can be individually charged, suggesting stable capacitance nanobits with a potential for information storage technology.