Preparation of IrO2-Ta2O5|Ti electrodes by immersion, painting and electrophoretic deposition for the electrochemical removal of hydrocarbons from water

After intense years of great development, the electrochemical technologies have become very suitable alternatives in niche markets like industrial wastewater reclamation and soil remediation. A key role to achieve a high efficiency in such treatments is played by the characteristics of the coating o...

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Detalles Bibliográficos
Autores: Herrada García, Rosa Alhelí, Medel, Alejandro, Manríquez, Federico, Sirés Sadornil, Ignacio, Bustos, Erika
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2016
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2445/168978
Acceso en línea:https://hdl.handle.net/2445/168978
Access Level:acceso abierto
Palabra clave:Oxidació electroquímica
Hidrocarburs
Depuració de l'aigua
Electrolytic oxidation
Hydrocarbons
Water purification
Descripción
Sumario:After intense years of great development, the electrochemical technologies have become very suitable alternatives in niche markets like industrial wastewater reclamation and soil remediation. A key role to achieve a high efficiency in such treatments is played by the characteristics of the coating of the electrodes employed. This paper compares three techniques, namely immersion, painting and electrophoresis, for the preparation of IrO2-Ta2O5|Ti, so-called dimensionally stable anodes (DSA®). The quality of the coatings has been investigated by means of surface and electrochemical analysis. Their ability to generate hydroxyl radicals and degrade aqueous solutions of hydrocarbons like phenanthrene, naphthalene and fluoranthene has been thoroughly assessed. Among the synthesis techniques, electrophoretic deposition yielded the best results, with DSA® electrodes exhibiting a homogeneous surface coverage that led to a good distribution of active sites, thus producing hydroxyl radicals that were able to accelerate the degradation of hydrocarbons.