Nonequilibrium plasmon emission drives ultrafast carrier relaxation dynamics in photoexcited graphene

The fast decay of carrier inversion in photoexcited graphene has been attributed to optical phonon emission and Auger recombination. Plasmon emission provides another pathway that, as we show here, drives the carrier relaxation dynamics on ultrafast time scales. In studying the nonequilibrium relaxa...

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Detalles Bibliográficos
Autores: Hamm, Joachim, Page, A. Freddie, Bravo Abad, Jorge, García Vidal, Fco. José, Hess, Ortwin G
Tipo de recurso: artículo
Fecha de publicación:2016
País:España
Institución:Universidad Autónoma de Madrid
Repositorio:Biblos-e Archivo. Repositorio Institucional de la UAM
Idioma:inglés
OAI Identifier:oai:repositorio.uam.es:10486/676766
Acceso en línea:http://hdl.handle.net/10486/676766
https://dx.doi.org/10.1103/PhysRevB.93.041408
Access Level:acceso abierto
Palabra clave:Photoexcited Graphene
Física
Descripción
Sumario:The fast decay of carrier inversion in photoexcited graphene has been attributed to optical phonon emission and Auger recombination. Plasmon emission provides another pathway that, as we show here, drives the carrier relaxation dynamics on ultrafast time scales. In studying the nonequilibrium relaxation dynamics we find that plasmon emission effectively converts inversion into hot carriers, whose energy is then extracted by optical phonon emission. This mechanism not only explains the observed femtosecond lifetime of inversion but also offers the prospect for atomically thin ultrafast plasmon emitters