Effect of catalytic graphitization on the electrochemical behavior of wood derived carbons for use in supercapacitors

© 2014 Elsevier B.V. All rights reserved. Porous graphitic carbons were successfully obtained from wood precursors through pyrolysis using a transition metal as catalyst. Once the catalyst is removed, the resulting material mimics the microstructure of the wood and presents high surface area, open a...

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Detalles Bibliográficos
Autores: Gutiérrez-Pardo, A., Ramírez-Rico, J., Cabezas-Rodríguez, R., Martínez-Fernández, Julián
Tipo de recurso: artículo
Fecha de publicación:2015
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/112799
Acceso en línea:http://hdl.handle.net/10261/112799
Access Level:acceso abierto
Palabra clave:Supercapacitors
Electrochemistry
Pyrolysis
Graphite
Carbon materials
Descripción
Sumario:© 2014 Elsevier B.V. All rights reserved. Porous graphitic carbons were successfully obtained from wood precursors through pyrolysis using a transition metal as catalyst. Once the catalyst is removed, the resulting material mimics the microstructure of the wood and presents high surface area, open and interconnected porosity and large pore volume, high crystallinity and good electrical conductivity, making these carbons interesting for electrochemical devices. Carbons obtained were studied as electrodes for supercapacitors in half cell experiments, obtaining high capacitance values in a basic media (up to 133 F g-1 at current densities of 20 mA g-1 and 35 F g-1 at current densities of 1 A g-1). Long-cycling experiments showed excellent stability of the electrodes with no reduction of the initial capacitance values after 1000 cycles in voltammetry.