Role of Polymorphism and Thin-Film Morphology in Organic Semiconductors Processed by Solution Shearing

Organic semiconductors (OSCs) are promising materials for costeffective production of electronic devices because they can be processed from solution employing high-throughput techniques. However, small-molecule OSCs are prone to structural modifications because of the presence of weak van der Waals...

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Detalles Bibliográficos
Autores: Riera Galindo, Sergi, Tamayo, Adrián, Mas Torrent, Marta
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2018
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/164403
Acceso en línea:http://hdl.handle.net/10261/164403
Access Level:acceso abierto
Palabra clave:Crystal structures
Deposition process
Phase transition
Polymer morphology
Descripción
Sumario:Organic semiconductors (OSCs) are promising materials for costeffective production of electronic devices because they can be processed from solution employing high-throughput techniques. However, small-molecule OSCs are prone to structural modifications because of the presence of weak van der Waals intermolecular interactions. Hence, controlling the crystallization in these materials is pivotal to achieve high device reproducibility. In this perspective article, we focus on controlling polymorphism and morphology in small-molecule organic semiconducting thin films deposited by solution-shearing techniques compatible with roll-to-roll systems. Special attention is paid to the influence that the different experimental deposition parameters can have on thin films. Further, the main characterization techniques for thin-film structures are reviewed, highlighting the in situ characterization tools that can provide crucial insights into the crystallization mechanisms.