Impedance spectroscopy of encapsulated single graphene layers

In this work, we demonstrate the use of electrical impedance spectroscopy (EIS) for the disentanglement of several dielectric contributions in encapsulated single graphene layers. The dielectric data strongly vary qualitatively with the nominal graphene resistance. In the case of sufficiently low re...

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Detalles Bibliográficos
Autores: Schmidt, Rainer, Carrascoso Plana, Félix, Nemes, Norbert Marcel, Mompeán, Federico, García-Hernández, Mar
Tipo de recurso: artículo
Fecha de publicación:2022
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/93789
Acceso en línea:https://hdl.handle.net/20.500.14352/93789
Access Level:acceso abierto
Palabra clave:538.9
Single-layer graphene
Impedance spectroscopy
Electrode resistance
Física del estado sólido
2211 Física del Estado Sólido
Descripción
Sumario:In this work, we demonstrate the use of electrical impedance spectroscopy (EIS) for the disentanglement of several dielectric contributions in encapsulated single graphene layers. The dielectric data strongly vary qualitatively with the nominal graphene resistance. In the case of sufficiently low resistance of the graphene layers, the dielectric spectra are dominated by inductive contributions, which allow for disentanglement of the electrode/graphene interface resistance from the intrinsic graphene resistance by the application of an adequate equivalent circuit model. Higher resistance of the graphene layers leads to predominantly capacitive dielectric contributions, and the deconvolution is not feasible due to the experimental high frequency limit of the EIS technique.