Influence of long-range atmospheric transport pathways and climate teleconnection patterns on the variability of surface Pb-210 and Be-7 concentrations in southwestern Europe

The variability of the atmospheric concentration of the 7Be and 210Pb radionuclides is strongly linked to the origin of air masses, the strength of their sources and the processes of wet and dry deposition. It has been shown how these processes and their variability are strongly affected by climate...

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Detalles Bibliográficos
Autores: Grossi, Claudia|||0000-0001-6678-4440, Ballester, Joan, Serrano Carreño, M. Isabel|||0000-0002-4996-9280, Galmarini, Stefano, Camacho García, Antonia|||0000-0003-2445-8326, Curcoll, Roger, Morguí, Josep Anton, Rodó, Xavier, Duch Guillen, María Amor|||0000-0002-1560-1576
Tipo de recurso: artículo
Fecha de publicación:2016
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/100962
Acceso en línea:https://hdl.handle.net/2117/100962
https://dx.doi.org/10.1016/j.jenvrad.2016.09.011
Access Level:acceso abierto
Palabra clave:Climatic changes - Península Ibèrica
Radioisotopes
Meteorology - Península Ibèrica
Be-7
Pb-210
WeMO
NAO
Climate
Air masses pathways
Canvis climàtics - Península Ibèrica
Isòtops radioactius
Meteorologia - Península Ibèrica
Àrees temàtiques de la UPC::Desenvolupament humà i sostenible::Degradació ambiental::Canvi climàtic
Àrees temàtiques de la UPC::Desenvolupament humà i sostenible::Degradació ambiental::Contaminació atmosfèrica
Descripción
Sumario:The variability of the atmospheric concentration of the 7Be and 210Pb radionuclides is strongly linked to the origin of air masses, the strength of their sources and the processes of wet and dry deposition. It has been shown how these processes and their variability are strongly affected by climate change. Thus, a deeper knowledge of the relationship between the atmospheric radionuclides variability measured close to the ground and these atmospheric processes could help in the analysis of climate scenarios. In the present study, we analyze the atmospheric variability of a 14-year time series of 7Be and 210Pb in a Mediterranean coastal city using a synergy of different indicators and tools such as: the local meteorological conditions, global and regional climate indexes and a lagrangian atmospheric transport model. We particularly focus on the relationships between the main pathways of air masses and sun spots occurrence, the variability of the local relative humidity and temperature conditions, and the main modes of regional climate variability, such as the North Atlantic Oscillation (NAO) and the Western Mediterranean Oscillation (WeMO). The variability of the observed atmospheric concentrations of both 7Be and 210Pb radionuclides was found to be mainly positively associated to the local climate conditions of temperature and to the pathways of air masses arriving at the station. Measured radionuclide concentrations significantly increase when air masses travel at low tropospheric levels from central Europe and the western part of the Iberian Peninsula, while low concentrations are associated with westerly air masses. We found a significant negative correlation between the WeMO index and the atmospheric variability of both radionuclides and no significant association was observed for the NAO index.