Multienzymatic platform for coupling a CCU strategy to waste valorization

Ongoing climate crisis demands the development of carbon capture and utilization (CCU) technologies that emphasize simplicity, eco-sustainability, and cost-effectiveness. Enzymatic CO2 reduction emerges as an alternative to biotransforming this cheap raw material into high-value products under milde...

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Detalles Bibliográficos
Autores: Rodriguez, Sady Roberto|||0000-0002-6035-6952, Álvaro, Gregorio|||0000-0002-2924-8902, Guillén, Marina|||0000-0002-9740-9966, Romero, Oscar|||0000-0002-0223-5167
Tipo de recurso: artículo
Fecha de publicación:2025
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:306528
Acceso en línea:https://ddd.uab.cat/record/306528
https://dx.doi.org/urn:doi:10.1021/acssuschemeng.4c04908
Access Level:acceso abierto
Palabra clave:CO2 reduction
Carbon Capture and Utilization
Waste valorization
Multienzymatic system
High-value chemicals
Descripción
Sumario:Ongoing climate crisis demands the development of carbon capture and utilization (CCU) technologies that emphasize simplicity, eco-sustainability, and cost-effectiveness. Enzymatic CO2 reduction emerges as an alternative to biotransforming this cheap raw material into high-value products under milder conditions. This work proposes a multienzymatic platform to reduce CO2 to formate by formate dehydrogenase (FDH) and oxidize glycerol to dihydroxyacetone (DHA) by glycerol dehydrogenase (GlyDH), allowing for efficient cofactor regeneration. Through studies such as pH operating range, enzyme stability, FDH/GlyDH ratio, and reaction medium engineering to achieve optimal soluble CO2 concentrations, the reaction with a gas mixture of 24% CO2 yielded 5.7 mM formate and 6 mM DHA after 30 h, achieving a 92.3% CO2 conversion. To evaluate the feasibility under industrially relevant conditions, a synthetic gas mixture mimicking the composition of the iron and steel industry off-gases (24.5% CO2) and crude glycerol (64% v/v) from biodiesel production was tested as substrates. The simultaneous production was successful, yielding 3.1 mM formate and 4.4 mM DHA. Formic acid was subsequently purified using liquid-liquid extraction, employing the green solvent 2-methyltetrahydrofuran (2-MTHF). For the first time to our knowledge, a CCU strategy has been successfully coupled with industrial waste valorization, obtaining two high-value molecules by means of a robust, profitable, and easily manageable multienzymatic system.