Solution-based synthesis and processing of Sn- and Bi-doped Cu₃SbSe₄ nanocrystals, nanomaterials and ring-shaped thermoelectric generators

Copper-based chalcogenides that comprise abundant, low-cost, and environmental friendly elements are excellent materials for a number of energy conversion applications, including photovoltaics, photocatalysis, and thermoelectrics (TE). In such applications, the use of solution-processed nanocrystals...

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Detalles Bibliográficos
Autores: Liu, Yu|||0000-0001-7313-6740, Ortega, Silvia|||0000-0002-3812-5146, Cadavid, Doris|||0000-0002-1376-6078, Ibáñez, Maria|||0000-0001-5013-2843, Xi, Lili, De Roo, Jonathan, López Peña, Antonio M.|||0000-0002-6979-5783, Martí-Sánchez, Sara|||0000-0003-4283-1489, Cabezas, Ignasi, De La Mata, Maria|||0000-0002-1581-4838, Luo, Zhishan|||0000-0002-0801-9238, Dun, Chaochao, Dobrozhan, Oleksandr|||0000-0001-9238-7596, Zhang, Wenqing, Martins, José, Kovalenko, Maksym V.|||0000-0002-6396-8938, Arbiol i Cobos, Jordi|||0000-0002-0695-1726, Noriega, German, Song, Ji-Ming, Cabot i Codina, Andreu|||0000-0002-7533-3251
Tipo de recurso: artículo
Fecha de publicación:2017
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:194415
Acceso en línea:https://ddd.uab.cat/record/194415
https://dx.doi.org/urn:doi:10.1039/c6ta08467b
Access Level:acceso abierto
Palabra clave:Bulk nano-materials
Composition control
Electronic band structure
Environmental-friendly
Lattice thermal conductivity
Solution-processing
Synthesis and processing
Thermoelectric generators
Descripción
Sumario:Copper-based chalcogenides that comprise abundant, low-cost, and environmental friendly elements are excellent materials for a number of energy conversion applications, including photovoltaics, photocatalysis, and thermoelectrics (TE). In such applications, the use of solution-processed nanocrystals (NCs) to produce thin films or bulk nanomaterials has associated several potential advantages, such as high material yield and throughput, and composition control with unmatched spatial resolution and cost. Here we report on the production of Cu₃SbSe₄ (CASe) NCs with tuned amounts of Sn and Bi dopants. After proper ligand removal, as monitored by nuclear magnetic resonance and infrared spectroscopy, these NCs were used to produce dense CASe bulk nanomaterials for solid state TE energy conversion. By adjusting the amount of extrinsic dopants, dimensionless TE figures of merit (ZT) up to 1.26 at 673 K were reached. Such high ZT values are related to an optimized carrier concentration by Sn doping, a minimized lattice thermal conductivity due to efficient phonon scattering at point defects and grain boundaries, and to an increase of the Seebeck coefficient obtained by a modification of the electronic band structure with Bi doping. Nanomaterials were further employed to fabricate ring-shaped TE generators to be coupled to hot pipes, which provided 20 mV and 1 mW per TE element when exposed to a 160 °C temperature gradient. The simple design and good thermal contact associated with the ring geometry and the potential low cost of the material solution processing may allow the fabrication of TE generators with short payback times.