Modelling of Optical Damage in Nanorippled ZnO Produced by Ion Irradiation

Here, we report on the production of nanoripples on the surface of ZnO bulk substrates by ion beam erosion with 20 keV Ar+ ions at an oblique incidence (60◦ ). The ripple patterns, analyzed by atomic force microscopy, follow a power law dependence for both the roughness and the wavelength. At high f...

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Detalles Bibliográficos
Autores: Redondo Cubero, Andrés, Vázquez Burgos, Luis Fernando, Jalabert, Denis, Lorenz, Katharina, Sedrine, Nabiha Ben
Tipo de recurso: artículo
Fecha de publicación:2019
País:España
Institución:Universidad Autónoma de Madrid
Repositorio:Biblos-e Archivo. Repositorio Institucional de la UAM
Idioma:inglés
OAI Identifier:oai:repositorio.uam.es:10486/714088
Acceso en línea:http://hdl.handle.net/10486/714088
https://dx.doi.org/10.3390/cryst9090453
Access Level:acceso abierto
Palabra clave:ZnO
patterning
sputtering
spectroscopic ellipsometry
ripples
damage
Física
Descripción
Sumario:Here, we report on the production of nanoripples on the surface of ZnO bulk substrates by ion beam erosion with 20 keV Ar+ ions at an oblique incidence (60◦ ). The ripple patterns, analyzed by atomic force microscopy, follow a power law dependence for both the roughness and the wavelength. At high fluences these ripples show coarsening and asymmetric shapes, which become independent of the beam direction and evidence additional mechanisms for the pattern development. The shallow damaged layer is not fully amorphized by this process, as confirmed by medium energy ion scattering. A detailed study of the damage-induced changes on the optical properties was carried out by means of spectroscopic ellipsometry. Using a 3-layer model based on Tauc-Lorenz and critical point parameter band oscillators, the optical constants of the damaged layer were determined. The results showed a progressive reduction in the refractive index and enhanced absorption below the bandgap with the fluence