Microflow Injection System for Efficient Cu(II) Detection across a Broad Range

In this study, a modular, multi-step, photometric microflow injection analysis (micro-FIA) system for the automatic determination of Cu(II) in a bioreactor was developed. The system incorporates diverse 3D-printed modules, including a platform formed by a mixer module to mix Cu(II) with hydroxylamin...

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Detalles Bibliográficos
Autores: Ricart, David, Dorado, Antonio David|||0000-0003-0238-5867, Lao-Luque, Conxita|||0000-0002-7342-7801, Baeza, Mireia|||0000-0002-2240-6410
Tipo de recurso: artículo
Fecha de publicación:2024
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:300962
Acceso en línea:https://ddd.uab.cat/record/300962
https://dx.doi.org/urn:doi:10.3390/chemosensors12070119
Access Level:acceso abierto
Palabra clave:3D-printed microfluidic platform
Cu(II)
Bioleaching
Circular economy
E-waste
Micro-fia
SDG 8 - Decent Work and Economic Growth
SDG 12 - Responsible Consumption and Production
Descripción
Sumario:In this study, a modular, multi-step, photometric microflow injection analysis (micro-FIA) system for the automatic determination of Cu(II) in a bioreactor was developed. The system incorporates diverse 3D-printed modules, including a platform formed by a mixer module to mix Cu(II) with hydroxylamine, which reduces Cu(II) to Cu(I) linked to a diluter module via a Tesla valve, a chelation mixer module, a disperser module, and a detector module provided by an LED light source at λ = 455 nm and a light dependence resistor (LDR) as a light intensity detector. The system measures the color intensity resulting from the chelation between Cu(I) and neocuproine. The micro-FIA system demonstrated good capability for automatic and continuous Cu(II) determination, in a wide range of Cu concentrations, from 34 to 2000 mg L -1. The device exhibits a good repeatability (coefficient of variation below 2% across the measured concentration range), good reproducibility, and has an accuracy of around 100% between 600 and 1900 mg L -1. Real samples were analyzed using both the micro-FIA system and an atomic absorption spectroscopy method, revealing no statistically significant differences. Additionally, a Tesla valve located before the detector substituted a 3-way solenoid valve, eliminating the need for moving parts.