Creep and recovery behavior of metallic glasses in a global strain approach within transition state theory

A unique global strain approach based on the transition state theory was proposed to quantify the creep-recovery processes of metallic glasses, in which the structure of glasses is predominantly governed by the macroscopic strain. This methodology allows for the calculation of strain-dependent activ...

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Bibliographic Details
Authors: Zhang, Langting, Duan, Yajuan, Wang, Yunjiang, Pineda Soler, Eloi|||0000-0002-1871-3848, Yang, Yong, Pelletier, Jean Marc, Wada, Takeshi, Kato, Hidemi, Crespo Artiaga, Daniel|||0000-0003-1743-2400, Qiao, Jichao
Format: article
Publication Date:2026
Country:España
Institution:Universitat Politècnica de Catalunya (UPC)
Repository:UPCommons. Portal del coneixement obert de la UPC
Language:English
OAI Identifier:oai:upcommons.upc.edu:2117/455609
Online Access:https://hdl.handle.net/2117/455609
https://dx.doi.org/10.1007/s10409-025-25311-x
Access Level:Embargoed access
Keyword:Metallic glass
Creep
Recovery
Anelasticity
Plasticity
Àrees temàtiques de la UPC::Enginyeria dels materials::Metal·lúrgia
Description
Summary:A unique global strain approach based on the transition state theory was proposed to quantify the creep-recovery processes of metallic glasses, in which the structure of glasses is predominantly governed by the macroscopic strain. This methodology allows for the calculation of strain-dependent activation energy and activation volume for flow defects. The activation energy and volume of creep both increase linearly with the magnitude of strain. Upon the glass-to-liquid transition, they get large and strain-independent, which serves as a signature of the glass transition. During creep recovery, the cooperation of deformation units increases the activation volume but decreases activation energy due to the decrease in free volume. Notably, only a fraction of the anelasticity accumulated during creep persists in the recovery process; the rest is suppressed by structural relaxation. The results introduce physical insights into the deformation and relaxation of metastable solids that are not available in the usual rate-dependent theory developed for crystal plasticity.