GdBO3 and YBO3 crystals under compression

[EN] High-pressure X-ray diffraction studies on nanocrystals of the GdBO3 and YBO3 rare-earth orthoborates are herein reported up to 17.4(2) and 13.4(2) GPa respectively. The subsequent determination of the room- temperature pressure-volume equations of state is presented and discussed in the contex...

Descripción completa

Detalles Bibliográficos
Autores: Turnbull, Robin, Errandonea, Daniel, Ibáñez, Jordi, Popescu, Catalin, Szczeszak, Agata, Lis, Stefan, Sans-Tresserras, Juan Ángel|||0000-0001-9047-3992, Cuenca-Gotor, Vanesa Paula|||0000-0003-0819-8528, Vilaplana Cerda, Rosario Isabel|||0000-0003-0504-2157, Manjón, Francisco-Javier|||0000-0002-3926-1705
Tipo de recurso: artículo
Fecha de publicación:2021
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/181738
Acceso en línea:https://riunet.upv.es/handle/10251/181738
Access Level:acceso abierto
Palabra clave:High-pressure
Synchrotron radiation
X-ray diffraction
Inelastic light scattering
Bulk modulus
Phosphors
FISICA APLICADA
Descripción
Sumario:[EN] High-pressure X-ray diffraction studies on nanocrystals of the GdBO3 and YBO3 rare-earth orthoborates are herein reported up to 17.4(2) and 13.4(2) GPa respectively. The subsequent determination of the room- temperature pressure-volume equations of state is presented and discussed in the context of contemporary publications which contradict the findings of this work. In particular, the isothermal bulk moduli of GdBO3 and YBO3 are found to be 170(13) and 163(13) GPa respectively, almost 50% smaller than recent findings. Our experimental results provide an accurate revision of the high-pressure compressibility behaviour of GdBO3 and YBO3 which is consistent with the known systematics in isomorphic borates and previous ab initio calculations. Finally, we discuss how experimental/analytical errors could have led to unreliable conclusions reported elsewhere.