Tailoring magnetization and anisotropy of tetragonal Mn3Ga thin films by strain-induced growth and spin orbit coupling

Tetragonal Mn3Ga thin films were epitaxially grown with and without strain on Cr and Mo crystalline buffer layers, respectively, using rf-magnetron sputtering. Epilayers grown on Cr with a lattice mismatch of 4.16%, exhibit a high magnetization of 220 kAm−1 and high perpendicular magnetic anisotropy...

Descripción completa

Detalles Bibliográficos
Autores: López Antón, Ricardo, Gutiérrez Pérez, Rocío Margarita, Załęski, Karol, Holguín Momaca, José Trinidad, Espinosa Magaña, Francisco, Olive Méndez, Sion Federico
Tipo de recurso: artículo
Fecha de publicación:2018
País:España
Institución:Universidad de Castilla-La Mancha
Repositorio:RUIdeRA. Repositorio Institucional de la UCLM
OAI Identifier:oai:ruidera.uclm.es:10578/18292
Acceso en línea:http://hdl.handle.net/10578/18292
Access Level:acceso abierto
Palabra clave:Thin films and multilayers
Magnetic properties
Deposition
Interfaces
Descripción
Sumario:Tetragonal Mn3Ga thin films were epitaxially grown with and without strain on Cr and Mo crystalline buffer layers, respectively, using rf-magnetron sputtering. Epilayers grown on Cr with a lattice mismatch of 4.16%, exhibit a high magnetization of 220 kAm−1 and high perpendicular magnetic anisotropy. These characteristics are attributed to interfacial strain. Additionally, a soft ferromagnetic component is observed in these films but not in relaxed layers grown on Mo, where Δa/a is −0.1%. These latest films exhibit a low magnetization of 80 kAm−1 and both perpendicular and in-plane magnetic anisotropies. We propose that high spin orbit coupling of Mo-5s14d5 orbitals from the buffer layer and strong hybridization with Mn3+-3d4 orbitals from the magnetic layer are at the origin of in-plane anisotropy at the interface, while Mn3Ga magnetocrystalline anisotropy leads to perpendicular anisotropy on the rest of the film.