Initial stages of the growth of mixed iron-cobalt oxides on Ru(0001)

Mixed iron-cobalt oxides have been grown on a Ru(0001) single crystal substrate by reactive molecular beam epitaxy. The growth has been followed by low-energy electron microscopy and diffraction. Chemical characterization has been performed by selected area x-ray absorption spectroscopy. As previous...

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Detalles Bibliográficos
Autores: Martín García, Laura, Quesadab, Adrian, Pérez García, Lucas, Foerster, Michael, Aballe, Lucía, Figuera, Juan de la
Tipo de recurso: artículo
Fecha de publicación:2016
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/23355
Acceso en línea:https://hdl.handle.net/20.500.14352/23355
Access Level:acceso abierto
Palabra clave:538.9
Cobalt monoxide
iron monoxide
Reactive molecular beam epitaxy
Low-energy electron microscopy
Selected area x-ray absorption
Photoemission electron microscopy
Física de materiales
Física del estado sólido
2211 Física del Estado Sólido
Descripción
Sumario:Mixed iron-cobalt oxides have been grown on a Ru(0001) single crystal substrate by reactive molecular beam epitaxy. The growth has been followed by low-energy electron microscopy and diffraction. Chemical characterization has been performed by selected area x-ray absorption spectroscopy. As previously known, iron grows into a wetting layer of FeO. In contrast, cobalt grows into three-dimensional islands of CoO, of either with a (111) –most common-or a (100) orientation. For mixed compositions, flat 2D growth is regained. Depending on temperature, either segregation into two FeCo compositions or a single phase is detected. In all cases the structure corresponds to an in-plane expanded (111)-oriented halite one. When only one phase is observed or for the Co-rich phase in the two phase film, its crystal structure is rotated by 30. relative to the Ru substrate, unlike the Co-poor phase which appears aligned with the substrate.