Exploration of magnetic order in Pr0.5Ca0.5CoO3-δ (δ=0) below the metal-insulator transition

We have investigated the low temperature magnetic state of Pr0.5Ca0.5CoO3-δ with (δ=0) by means of resistivity, dc magnetization, susceptibility, magnetotransport and neutron diffraction. We find that below the metal-insulator transition (MIT) this system can be described as a paramagnetic insulator...

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Detalles Bibliográficos
Autores: Barón González, Aura J., Frontera, Carlos, García Muñoz, Josep Lluís, Blasco, Javier, Ritter, C., Valencia, Sergio, Feyerhermd, R., Dudzik, Esther
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2010
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/367303
Acceso en línea:http://hdl.handle.net/10261/367303
Access Level:acceso abierto
Palabra clave:Magnetic order
Metal-insulator transition
Cobaltites
Perovskites
Descripción
Sumario:We have investigated the low temperature magnetic state of Pr0.5Ca0.5CoO3-δ with (δ=0) by means of resistivity, dc magnetization, susceptibility, magnetotransport and neutron diffraction. We find that below the metal-insulator transition (MIT) this system can be described as a paramagnetic insulator with dominant ferromagnetic interactions between Co atoms. In this regime, it presents a considerable negative magnetoresistance (20%-40%), while above MIT the magnetoresistance is negligible or even slightly positive. Neutron diffraction measurements reveal that there is no long-range ferromagnetic (FM) or antiferromagnetic (AFM) order. These results are in contradiction with the spin state picture previously drawn for this system.