Circularly Polarized Attosecond Pulses Enabled by an Azimuthal Phase and Polarization Grating

[EN]High-harmonic generation (HHG) is an extreme nonlinear optical process that can map the properties of an infrared driving laser beam onto short wavelength attosecond pulse trains. However, current techniques for generating circularly polarized high harmonics for probing magnetic materials and ch...

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Detalles Bibliográficos
Autores: Brooks, Nathan J., Heras, Alba de las, Wang, Bin, Binnie, Iona, Serrano, Javier, San Román Álvarez de Lara, Julio, Plaja Rustein, Luis, Kapteyn, Henry C., Hernández García, Carlos, Murnane, Margaret M.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2024
País:España
Institución:Universidad de Salamanca (USAL)
Repositorio:GREDOS. Repositorio Institucional de la Universidad de Salamanca
OAI Identifier:oai:gredos.usal.es:10366/168575
Acceso en línea:http://hdl.handle.net/10366/168575
Access Level:acceso abierto
Palabra clave:High-harmonic generation
Attosecond science
Extreme ultraviolet
Soft X-ray
Structured light
Optical vortices
Descripción
Sumario:[EN]High-harmonic generation (HHG) is an extreme nonlinear optical process that can map the properties of an infrared driving laser beam onto short wavelength attosecond pulse trains. However, current techniques for generating circularly polarized high harmonics for probing magnetic materials and chiral systems have limitations: two-color collinear counter-rotating driving lasers result in a low cutoff photon energy, while single-color noncollinear counter-rotating schemes suffer from low conversion efficiency. In this work, we generate circularly polarized attosecond pulse trains by using a structured laser driver which has a rotating polarization and phase grating along the azimuthal coordinate. Our experimental and numerical results demonstrate the production of left and right circularly polarized harmonics, which naturally separate upon propagation. Our approach uses a single laser color in a collinear geometry, that can be scaled for high efficiency. Simulations show this scheme can extend into the soft X-ray region when driven by mid-infrared driving lasers, while preserving the same high phase-matching cutoff photon energy as for linearly polarized high harmonics.