Electrochemical lossy mode resonance for detection of manganese ions

In this work we propose electrochemical lossy mode resonance (eLMR) as a powerful method for the detection of manganese (Mn) ions. The sensor is based on a simple planar waveguide (sodasingle bondlime glass coverslip) coated with a thin layer of indium tin oxide (ITO) to obtain an optical resonance...

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Detalles Bibliográficos
Autores: Domínguez Rodríguez, Ismel, Corres Sanz, Jesús María, Villar Fernández, Ignacio del, Mozo Llamazares, Juan Daniel, Simerova, Radka, Sezemsky, Petr, Stranak, Vitezslav, Smietana, Mateusz, Matías Maestro, Ignacio Raúl
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universidad de Huelva (UHU)
Repositorio:Arias Montano. Repositorio Institucional de la Universidad de Huelva
Idioma:inglés
OAI Identifier:oai:ariasmontano.uhu.es:10272/23928
Acceso en línea:https://hdl.handle.net/10272/23928
Access Level:acceso abierto
Palabra clave:Optical sensing
Electrochemical sensing
Heavy metal ions detection
Thin-film
Indium tin oxide
Lossy mode resonance
Stripping voltammetry
3303 Ingeniería y Tecnología Químicas
Descripción
Sumario:In this work we propose electrochemical lossy mode resonance (eLMR) as a powerful method for the detection of manganese (Mn) ions. The sensor is based on a simple planar waveguide (sodasingle bondlime glass coverslip) coated with a thin layer of indium tin oxide (ITO) to obtain an optical resonance effect. Simultaneously, the ITO layer served as the working electrode in the cathodic stripping voltammetry (CSV) of Mn. The eLMR sensor is capable of simultaneously performing electrochemical (EC) and optical measurements, specifically lossy mode resonance (LMR), to monitor the growth of the adsorbed Mn layer on the ITO electrode and the electrochemically modulated diffusion layer. For Mn2+ ions, a limit of detection (LoD) of 1.26 ppb has been demonstrated using the EC method, whereas the optical method exhibited a LoD of 67.76 ppb. The results obtained indicate significant potential for application in molecular electrochemistry and studies focused on electrified interfaces.