The proton binding properties of biosorbents

A broad variety of materials of biological origin have been successfully used in recent decades for the removal of pollutants from waters. These biosorbents include natural polymers that play a key role for adsorption. It is therefore critical to understand the physicochemical properties of the chem...

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Detalles Bibliográficos
Autores: Lodeiro, Pablo, Martínez-Cabanas, María, Herrero, Roberto, Barriada, José Luis, Vilariño, Teresa, Rodríguez-Barro, Pilar, Sastre de Vicente, Manuel E.
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2019
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:10459.1/71041
Acceso en línea:https://doi.org/10.1007/s10311-019-00883-z
http://hdl.handle.net/10459.1/71041
Access Level:acceso abierto
Palabra clave:Biosorption
Proton binding
Master curve
Electrostatics and non-electrostatic effects
Hofmeister series
Descripción
Sumario:A broad variety of materials of biological origin have been successfully used in recent decades for the removal of pollutants from waters. These biosorbents include natural polymers that play a key role for adsorption. It is therefore critical to understand the physicochemical properties of the chemical groups of these biopolymers. The acid-base properties of biomass are affected by pH, ionic strength and medium composition. Nevertheless, these parameters are not always considered during biosorption studies. According to the literature, less than 3% of biosorption reports include studies on proton binding. Moreover, in 60% of these papers, there is key experimental information missing such as the calibration of the electrodes employed for potentiometric titrations. We consider therefore that there is an important need for reviewing the role of proton binding in biosorption studies. This review outlines the major advances on data interpretation and modelling of proton binding on biosorbents. In addition, we discuss issues concerning the acid-base properties of biosorbents.