239PU, 240PU, and 241AM Determination in Hot Particles by Low Level Gamma-Spectrometry

A nondestructive method based on low-energy, highresolution photon spectrometry is presented which allows accurate determination of 239Pu, 240Pu, and 241Am (as a daughter of 241Pu) activities in radioactive particles containing relatively high levels of plutonium isotopes. The proposed method requir...

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Detalles Bibliográficos
Autores: Jiménez Ramos, María del Carmen, Hurtado Bermúdez, Santiago José, Chamizo, E., García-Tenorio García-Balmaseda, Rafael, León Vintró, Luis, Mitchell, P. I.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2010
País:España
Institución:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/146259
Acceso en línea:https://hdl.handle.net/11441/146259
https://doi.org/10.1021/es100425x
Access Level:acceso abierto
Palabra clave:Gamma-Spectrometry
Descripción
Sumario:A nondestructive method based on low-energy, highresolution photon spectrometry is presented which allows accurate determination of 239Pu, 240Pu, and 241Am (as a daughter of 241Pu) activities in radioactive particles containing relatively high levels of plutonium isotopes. The proposed method requires only one measurement for the establishment of an absolute efficiency curve. Since the density and composition of the radioactive particles of interest may vary, a self-absorption correction is required for the accurate determination of isotopic activities and ratios. This correction is carried out for each individual particle using the convenient gamma-ray emissions of 241 Am.