Intrinsic correlation between the fraction of liquidlike zones and the beta relaxation in high-entropy metallic glasses

Lacking the structural information of crystalline solids, the origin of the relaxation dynamics of metallic glasses is unclear. Here, we report the evolution of stress relaxation of high-entropy metallic glasses with distinct ß relaxation behavior. The fraction of liquidlike zones, determined at eac...

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Detalles Bibliográficos
Autores: Duan, Yajuan, Zhang, Langting, Qiao, J. C., Wang, Yun-Jiang, Yang, Y., Wada, T., Kato, Hidemi, Pelletier, J. M., Pineda Soler, Eloi|||0000-0002-1871-3848, Crespo Artiaga, Daniel|||0000-0003-1743-2400
Tipo de recurso: artículo
Fecha de publicación:2022
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/380615
Acceso en línea:https://hdl.handle.net/2117/380615
https://dx.doi.org/10.1103/PhysRevLett.129.175501
Access Level:acceso abierto
Palabra clave:Glass
Metallic glasses
Liquid metals
Glasses
Vidre
Vidres metàl·lics
Metalls líquids
Àrees temàtiques de la UPC::Física
Descripción
Sumario:Lacking the structural information of crystalline solids, the origin of the relaxation dynamics of metallic glasses is unclear. Here, we report the evolution of stress relaxation of high-entropy metallic glasses with distinct ß relaxation behavior. The fraction of liquidlike zones, determined at each temperature by the intensity of stress decay, is shown to be directly related to both the aging process and the spectrum of relaxation modes obtained by mechanical spectroscopy. The results shed light on the intrinsic correlation between the static and dynamic mechanical response in high-entropy and conventional metallic glasses, pointing toward a sluggish diffusion high-entropy effect in the liquid dynamics.