Photocontrolled strain in polycrystalline ferroelectrics via domain engineering strategy

The use of photonic concepts to achieve nanoactuation based on light triggering requires complex architectures to obtain the desired effect.In thiscontext, the recent discoveryof reversible optical control of the domain configurationin ferroelectricsoffers anew light-ferroic interplaythat can be eas...

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Detalhes bibliográficos
Autores: Rubio Marcos, Fernando, Del Campo Garcia, Angel Adolfo, Ordoñez Pimentel, Jonathan, Venet, Michel, Rojas Hernández, Rocio E., Páez Margarit, David, Ochoa Guerrero, Diego A.|||0000-0002-8756-9704, Fernández Lozano, José Francisco, García García, José Eduardo|||0000-0002-1232-1739
Formato: artículo
Fecha de publicación:2021
País:España
Recursos:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/345488
Acesso em linha:https://hdl.handle.net/2117/345488
https://dx.doi.org/10.1021/acsami.1c03162
Access Level:acceso abierto
Palavra-chave:Electrical engineering -- Materials
Photoferroelectrics
barium titanate
ferroelectric domains
photo-induced strain
light-induced phenomena
Ferroelectricitat
Ferroelectricitat -- Materials
Enginyeria elèctrica -- Materials
Àrees temàtiques de la UPC::Enginyeria dels materials::Materials funcionals::Materials elèctrics i electrònics
Descrição
Resumo:The use of photonic concepts to achieve nanoactuation based on light triggering requires complex architectures to obtain the desired effect.In thiscontext, the recent discoveryof reversible optical control of the domain configurationin ferroelectricsoffers anew light-ferroic interplaythat can be easily controlled. To date, however, the optical control of ferroelectric domains is explored insingle crystals, although polycrystals are technologically more desirable because they can be manufactured in a scalable and reproducible fashion. Here we report experimental evidencesfora large photo-strain response in polycrystalline BaTiO3that is comparable to theirelectro-strain values. Domainsengineering is performed through grain size control, thereby evidencing that charged domain walls appear to be the functional interfaces for the light-driven domain switching. Thefindingsshed light onthe design of high-performance photo-actuatorsbased on ferroelectric ceramics, providing afeasible alternativeto the conventional voltage-driven nanoactuators