Tunable high-field magnetization in strongly exchange-coupled freestanding Co/CoO core/shell coaxial nanowires

The exchange bias properties of Co/CoO coaxial core/shell nanowires have been investigated with cooling and applied fields perpendicular to the wire axis. This configuration leads to unexpected exchange-bias effects. Firstly, the magnetization value at high fields is found to depend on the field-coo...

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Detalles Bibliográficos
Autores: Salazar Álvarez, Germán|||0000-0002-0671-435X, Geshev, Julian|||0000-0003-3730-3657, Agramunt Puig, Sebastià|||0000-0002-3627-2820, Navau, Carles|||0000-0003-4763-5305, Sánchez Moreno, Álvaro|||0000-0002-2988-0289, Sort, Jordi|||0000-0003-1213-3639, Nogués, Josep|||0000-0003-4616-1371
Tipo de recurso: artículo
Fecha de publicación:2016
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:170261
Acceso en línea:https://ddd.uab.cat/record/170261
https://dx.doi.org/urn:doi:10.1021/acsami.6b05588
Access Level:acceso abierto
Palabra clave:Coaxial nanowires
Exchange bias
CoO
Uncopmpensated spins
Training effects
High field irreversibility
Descripción
Sumario:The exchange bias properties of Co/CoO coaxial core/shell nanowires have been investigated with cooling and applied fields perpendicular to the wire axis. This configuration leads to unexpected exchange-bias effects. Firstly, the magnetization value at high fields is found to depend on the field-cooling conditions. This effect arises from the competition between the magnetic anisotropy and the Zeeman energies for cooling fields perpendicular to the wire axis. This allows imprinting pre-defined magnetization states to the AFM, as corroborated by micromagnetic simulations. Secondly, the system exhibits a high-field magnetic irreversibility, leading to open hysteresis loops, attributed to the AFM easy-axis reorientation during the reversal (effect similar to athermal training). A distinct way to manipulate the high-field magnetization in exchange-biased systems, beyond the archetypical effects, is thus experimentally and theoretically demonstrated.