Time-resolved solvation of alkali ions in superfluid helium nanodroplets

The sinking of alkali cations in superfluid 4He nanodroplets is investigated theoretically using liquid 4He time-dependent density functional theory at zero temperature. The simulations illustrate the dynamics of the buildup of the first solvation shell around the ions. The number of helium atoms in...

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Detalles Bibliográficos
Autores: García-Alfonso, Ernesto, Barranco Gómez, Manuel, Halberstadt, Nadine, Pi Pericay, Martí
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2024
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2445/215902
Acceso en línea:https://hdl.handle.net/2445/215902
Access Level:acceso abierto
Palabra clave:Solvatació
Superfluïdesa
Heli
Solvation
Superfluidity
Helium
Descripción
Sumario:The sinking of alkali cations in superfluid 4He nanodroplets is investigated theoretically using liquid 4He time-dependent density functional theory at zero temperature. The simulations illustrate the dynamics of the buildup of the first solvation shell around the ions. The number of helium atoms in this shell is found to linearly increase with time during the first stages of the dynamics. This points to a Poissonian capture process, as concluded in the work of Albrechtsen <em>et al. </em>on the primary steps of Na+ solvation in helium droplets [Albrechtsen <em>et al.</em>, Nature <strong>623</strong>, 319 (2023)]. The energy dissipation rate by helium atom ejection is found to be quite similar between all alkalis, the main difference being a larger energy dissipated per atom for the lighter alkalis at the beginning of the dynamics. In addition, the number of helium atoms in the first solvation shell is found to be lower at the end of the dynamics than at equilibrium for both Li+ and Na+, pointing to a kinetic rather than thermodynamical control of the snowball size for small and strongly attractive ions.