Molecular dynamics data for modelling the microstructural behaviour of compacted sodium bentonites

The water retention curve deduced with low water content data allows the modelling of the bentonite void ratio associated with the pores located inside the clay aggregates, or micropores. However, if both the water content and the microporosity continue to increase, the latter can no longer be direc...

ver descrição completa

Detalhes bibliográficos
Autores: Navarro Gamir, Vicente, Yustres Real, Ángel, Jennis, Andrea, De la Morena, Gema, Asensio, Laura, López-Vizcaino López, Rubén, Cabrera, Virginia, Wersin, Paul, Mäders, Urs, Muuri, Eveliina, Niskanen, Mika, Akinwunmi, Bukunmi, Hirvi, Janne T., Pakkanen, Tapani A.
Tipo de documento: artigo
Data de publicação:2020
País:España
Recursos:Universidad de Castilla-La Mancha
Repositório:RUIdeRA. Repositorio Institucional de la UCLM
OAI Identifier:oai:ruidera.uclm.es:10578/27166
Acesso em linha:https://doi.org/10.1016/j.clay.2020.105932
http://hdl.handle.net/10578/27166
Access Level:Acceso aberto
Palavra-chave:Sodium bentonite
Continuum modelling
Molecular dynamics
Microstructural void ratio
Descrição
Resumo:The water retention curve deduced with low water content data allows the modelling of the bentonite void ratio associated with the pores located inside the clay aggregates, or micropores. However, if both the water content and the microporosity continue to increase, the latter can no longer be directly obtained from the former, because, in that case, the presence of water in the pores existing between the aggregates (macropores) may not be negligible. Therefore, it is not easy to obtain experimental evidence that allows to contrast whether the model's extrapolation of the microstructural void ratio obtained under dry conditions is valid for higher water contents. This work analyses the use of data obtained from molecular dynamics models to assess the validity of such extrapolations, and defines the variables needed to compare the results from molecular dynamics and laboratory experiments. The encouraging agreement obtained contributed to the confidence in the proposed procedure, which enabled a new strategy that uses molecular dynamics data to model the macroscopic behaviour of compacted sodium bentonites.