Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection

Traditionally, the nanoscale interaction between single photon emitters and plasmonic nanostructures is studied by relying on deterministic, near-perfect, nanoscale-control, either top-down or bottom-up. However, these approaches are ultra-low throughput thus rendering systematic studies difficult a...

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Detalhes bibliográficos
Autores: Saemisch, Lisa, Liebel, Matz, Hulst, Niek van
Formato: artículo
Fecha de publicación:2020
País:España
Recursos:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/192976
Acesso em linha:https://hdl.handle.net/2117/192976
https://dx.doi.org/10.1039/c9nr08833d
Access Level:acceso abierto
Palavra-chave:Optical antennas
nanoantennas
Antenes òptiques
Àrees temàtiques de la UPC::Física
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spelling Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detectionSaemisch, LisaLiebel, MatzHulst, Niek vanOptical antennasnanoantennasAntenes òptiquesÀrees temàtiques de la UPC::FísicaTraditionally, the nanoscale interaction between single photon emitters and plasmonic nanostructures is studied by relying on deterministic, near-perfect, nanoscale-control, either top-down or bottom-up. However, these approaches are ultra-low throughput thus rendering systematic studies difficult and timeconsuming. Here, we show a highly parallelised far-field tactic, combining multiplexed super-resolution fluorescence localization microscopy and data-driven statistical analysis, to study near-field interactions between gold nanorods and single molecules, even at bulk concentrations. We demonstrate that ensemble-level single molecule detection allows separating individual emitters according to their coupling strength with tailored resonant structures, which ultimately permits the reconstruction of super-resolved 2D interaction maps around individual nanoantennas.Peer ReviewedRoyal Society of Chemistry20202020-01-1620202020-07-15journal articlehttp://purl.org/coar/resource_type/c_6501AMhttp://purl.org/coar/version/c_ab4af688f83e57aainfo:eu-repo/semantics/articleapplication/pdfhttps://hdl.handle.net/2117/192976https://dx.doi.org/10.1039/c9nr08833dreponame:UPCommons. Portal del coneixement obert de la UPCinstname:Universitat Politècnica de Catalunya (UPC)InglésengEuropean Commission http://doi.org/10.13039/100010661 Horizon 2020 Framework Programme 670949 LightNetopen accesshttp://purl.org/coar/access_right/c_abf2Attribution-NonCommercial-NoDerivs 3.0 Spainhttp://creativecommons.org/licenses/by-nc-nd/3.0/es/info:eu-repo/semantics/openAccessoai:upcommons.upc.edu:2117/1929762026-05-27T15:37:01Z
dc.title.none.fl_str_mv Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
title Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
spellingShingle Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
Saemisch, Lisa
Optical antennas
nanoantennas
Antenes òptiques
Àrees temàtiques de la UPC::Física
title_short Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
title_full Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
title_fullStr Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
title_full_unstemmed Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
title_sort Isolating strong nanoantenna-molecule interactions by ensemble-level single-molecule detection
dc.creator.none.fl_str_mv Saemisch, Lisa
Liebel, Matz
Hulst, Niek van
author Saemisch, Lisa
author_facet Saemisch, Lisa
Liebel, Matz
Hulst, Niek van
author_role author
author2 Liebel, Matz
Hulst, Niek van
author2_role author
author
dc.subject.none.fl_str_mv Optical antennas
nanoantennas
Antenes òptiques
Àrees temàtiques de la UPC::Física
topic Optical antennas
nanoantennas
Antenes òptiques
Àrees temàtiques de la UPC::Física
description Traditionally, the nanoscale interaction between single photon emitters and plasmonic nanostructures is studied by relying on deterministic, near-perfect, nanoscale-control, either top-down or bottom-up. However, these approaches are ultra-low throughput thus rendering systematic studies difficult and timeconsuming. Here, we show a highly parallelised far-field tactic, combining multiplexed super-resolution fluorescence localization microscopy and data-driven statistical analysis, to study near-field interactions between gold nanorods and single molecules, even at bulk concentrations. We demonstrate that ensemble-level single molecule detection allows separating individual emitters according to their coupling strength with tailored resonant structures, which ultimately permits the reconstruction of super-resolved 2D interaction maps around individual nanoantennas.
publishDate 2020
dc.date.none.fl_str_mv 2020
2020-01-16
2020
2020-07-15
dc.type.none.fl_str_mv journal article
http://purl.org/coar/resource_type/c_6501
AM
http://purl.org/coar/version/c_ab4af688f83e57aa
dc.type.openaire.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv https://hdl.handle.net/2117/192976
https://dx.doi.org/10.1039/c9nr08833d
url https://hdl.handle.net/2117/192976
https://dx.doi.org/10.1039/c9nr08833d
dc.language.none.fl_str_mv Inglés
eng
language_invalid_str_mv Inglés
language eng
dc.relation.none.fl_str_mv European Commission http://doi.org/10.13039/100010661 Horizon 2020 Framework Programme 670949 LightNet
dc.rights.none.fl_str_mv open access
http://purl.org/coar/access_right/c_abf2
Attribution-NonCommercial-NoDerivs 3.0 Spain
http://creativecommons.org/licenses/by-nc-nd/3.0/es/
dc.rights.openaire.fl_str_mv info:eu-repo/semantics/openAccess
rights_invalid_str_mv open access
http://purl.org/coar/access_right/c_abf2
Attribution-NonCommercial-NoDerivs 3.0 Spain
http://creativecommons.org/licenses/by-nc-nd/3.0/es/
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.publisher.none.fl_str_mv Royal Society of Chemistry
publisher.none.fl_str_mv Royal Society of Chemistry
dc.source.none.fl_str_mv reponame:UPCommons. Portal del coneixement obert de la UPC
instname:Universitat Politècnica de Catalunya (UPC)
instname_str Universitat Politècnica de Catalunya (UPC)
reponame_str UPCommons. Portal del coneixement obert de la UPC
collection UPCommons. Portal del coneixement obert de la UPC
repository.name.fl_str_mv
repository.mail.fl_str_mv
_version_ 1869407708847800320
score 15.301603

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