Modified carbon fabric electrodes: preparation and electrochemical behavior toward amaranth electrolysis

The electrochemical behavior of non-modified, Pt-modified, and Pt/polyaniline-modified carbon fiber textile electrodes was studied through a series of electrolyses, under potentiostatic conditions, on an amaranth/sulfuric solution in the presence or absence of chloride ion. The morphology of the dis...

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Detalhes bibliográficos
Autores: Fernández Sáez, Javier, Del Río García, Ana Isabel, Molina Puerto, Javier|||0000-0003-3378-8271, Bonastre Cano, José Antonio|||0000-0002-5068-6608, Cases, Francisco|||0000-0001-8105-4489
Formato: artículo
Fecha de publicación:2015
País:España
Recursos:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/52203
Acesso em linha:https://riunet.upv.es/handle/10251/52203
Access Level:acceso abierto
Palavra-chave:Carbon fabric electrodes
Dispersed platinum
Polyaniline
Amaranth electrolysis
QUIMICA FISICA
Descrição
Resumo:The electrochemical behavior of non-modified, Pt-modified, and Pt/polyaniline-modified carbon fiber textile electrodes was studied through a series of electrolyses, under potentiostatic conditions, on an amaranth/sulfuric solution in the presence or absence of chloride ion. The morphology of the dispersed Pt, PANI, and PANI/Pt coatings was analyzed by scanning electron microscopy. Scanning electrochemical microscopy confirmed that the textile surface was effectively modified by the electrocatalytic material. Color removal reached values above 90 % in both electroreduction and electrooxidation processes. The amaranth electroreductions carried out with the non-modified electrode showed better charge efficiency than those with the Pt-modified textile electrode. The electrooxidations with Pt-modified textile electrodes showed a significant reduction in electrolysis time. Ultraviolet-visible and Fourier transform infrared with attenuated total reflection spectra enabled the electrochemical behavior of the non-modified and Pt/PANI-modified electrodes to be distinguished.