Simultaneous determination of organotin compounds by hydride generation-gas phase molecular absorption spectrometry

This study describes the determination of ternary mixtures of dimethyltin chloride (DMT), trimethyltin chloride (TMT) and monobutyltin chloride (BT) by hydride generation-gas phase molecular absorption spectrometry and the application of different chemometric methods: principal components regression...

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Detalles Bibliográficos
Autores: Sanz-Asensio, J., Martínez-Soria, M.T. [0000-0003-4208-2801], Plaza-Medina, M., Pérez Clavijo, M.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2001
País:España
Institución:Universidad de La Rioja (UR)
Repositorio:RIUR. Repositorio Institucional de la Universidad de La Rioja
OAI Identifier:oai:portal.dialnet.es:doc/5bbc69d3b750603269e8221e
Acceso en línea:https://investigacion.unirioja.es/documentos/5bbc69d3b750603269e8221e
Access Level:acceso abierto
Palabra clave:Gas phase molecular absorption spectrometry
Hydride generation
Organotin compounds
Descripción
Sumario:This study describes the determination of ternary mixtures of dimethyltin chloride (DMT), trimethyltin chloride (TMT) and monobutyltin chloride (BT) by hydride generation-gas phase molecular absorption spectrometry and the application of different chemometric methods: principal components regression (PCR) and partial least squares (PLS). The two methods are applied to the absorption spectra of mixtures of DMT, TMT and BT. Two different experimental designs are tested for the mixtures, a triangular design and a central composite design. The models obtained from the triangular design offer the best prediction results. The effects of the number of working wavelengths and the number of factors included in the calibration model is studied and a different behaviour is seen for each compound and calibration model. The methods are applied to the analysis of artificial aqueous samples containing different concentrations of DMT, TMT and BT species. No significant differences are observed between the calibration models investigated. © 2001 Elsevier Science B.V.