Molecular features of non-selective small molecule antagonists of the Bradykinin receptors

Angiotensin converting enzyme 2 (ACE2) downregulation is a key negative factor for the severity of lung edema and acute lung failure observed in patients infected with SARS-CoV-2. ACE2 downregulation affects the levels of diverse peptide mediators of the renin-agiotensin-aldestosterone and kallikrei...

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Detalles Bibliográficos
Autores: Rasaeifar, Bahareh, Gómez Gutierrez, Patricia, Pérez González, Juan Jesús|||0000-0002-0748-8147
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/334784
Acceso en línea:https://hdl.handle.net/2117/334784
https://dx.doi.org/10.3390/ph13090259
Access Level:acceso abierto
Palabra clave:COVID-19 (Disease)
Bradykinin receptors
Bradykinin pharmacophore
Non-peptide bradykinin antagonists
Bradykinin repurposing
Covid-19 therapy
COVID-19 (Malaltia)
Molècules
Àrees temàtiques de la UPC::Enginyeria química
Descripción
Sumario:Angiotensin converting enzyme 2 (ACE2) downregulation is a key negative factor for the severity of lung edema and acute lung failure observed in patients infected with SARS-CoV-2. ACE2 downregulation affects the levels of diverse peptide mediators of the renin-agiotensin-aldestosterone and kallikrein-kinin systems, compromising vascular hemostasis. Increasing evidence suggests that the inflammatory response observed in covid-19 patients is initiated by the action of kinins on the bradykinin receptors. Accordingly, the use of bradykinin antagonists should be considered as a strategy for therapeutic intervention against covid-19 illness progression. Presently, icatibant is the only bradykinin antagonist drug approved. In the present report, we investigated the molecular features characterizing non-selective antagonists targeting the bradykinin receptors and carried out a in silico screening of approved drugs, aimed at the identification of compounds with a non-selective bradykinin antagonist profile that can be evaluated for drug repurposing. The study permitted to identify eight compounds as prospective non-selective antagonists of the bradykinin receptors, including raloxifene; sildenafil; cefepime; cefpirome; imatinib; ponatinib; abemaciclib and entrectinib.