Detection of silver nanoparticles in seawater at ppb levels using UV-visible spectrophotometry with long path cells

Silver nanoparticles (AgNPs) are emerging contaminants that are difficult to detect in natural waters. UV-visible spectrophotometry is a simple technique that allows detection of AgNPs through analysis of their characteristic surface plasmon resonance band. The detection limit for nanoparticles usin...

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Detalles Bibliográficos
Autores: Lodeiro, Pablo, Achterberg, Eric P., El-Shahawi, Mohammad S.
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2017
País:España
Institución:Universitat de Lleida (UdL)
Repositorio:Repositori Obert UdL
OAI Identifier:oai:repositori.udl.cat:10459.1/71098
Acceso en línea:https://doi.org/10.1016/j.talanta.2016.11.055
http://hdl.handle.net/10459.1/71098
Access Level:acceso abierto
Palabra clave:Silver nanoparticles
Seawater
NM300K
Surface plasmon resonance band
UV–visible spectrophotometry
Long path cell
Descripción
Sumario:Silver nanoparticles (AgNPs) are emerging contaminants that are difficult to detect in natural waters. UV-visible spectrophotometry is a simple technique that allows detection of AgNPs through analysis of their characteristic surface plasmon resonance band. The detection limit for nanoparticles using up to 10 cm path length cuvettes with UV-visible spectrophotometry is in the 0.1-10 ppm range. This detection limit is insufficiently low to observe AgNPs in natural environments. Here we show how the use of capillary cells with an optical path length up to 200 cm, forms an excellent technique for rapid detection and quantification of non-aggregated AgNPs at ppb concentrations in complex natural matrices such as seawater.