Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts
The electrochemical CO2 reduction reaction (CO2RR) either to generate multicarbon (C2+) or single carbon (C1) value-added products provides an effective and promising approach to mitigate the high CO2 concentration in the atmosphere and promote energy storage. However, cost-effectiveness of catalyti...
| Autores: | , , , |
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| Formato: | artículo |
| Fecha de publicación: | 2020 |
| País: | España |
| Recursos: | Universidad de Cantabria (UC) |
| Repositorio: | UCrea Repositorio Abierto de la Universidad de Cantabria |
| Idioma: | inglés |
| OAI Identifier: | oai:repositorio.unican.es:10902/20736 |
| Acesso em linha: | http://hdl.handle.net/10902/20736 |
| Access Level: | acceso abierto |
| Palavra-chave: | Carbon dioxide electrochemical reduction reaction Electrocatalysis Oxide-derived copper catalysts Transition metal–nitrogen–carbon catalysts Value-added products |
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Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalystsElectrochemical CO2 reduction reaction on copper oxides and metal-nitrogen- carbon catalysts for value-added products generationZhang, LinMerino García, IvánAlbo Sánchez, Jonathan|||0000-0001-6781-5704Sánchez Sánchez, Carlos ManuelCarbon dioxide electrochemical reduction reactionElectrocatalysisOxide-derived copper catalystsTransition metal–nitrogen–carbon catalystsValue-added productsThe electrochemical CO2 reduction reaction (CO2RR) either to generate multicarbon (C2+) or single carbon (C1) value-added products provides an effective and promising approach to mitigate the high CO2 concentration in the atmosphere and promote energy storage. However, cost-effectiveness of catalytic materials limits practical application of this technology in the short term. Herein, we summarize and discuss recent and advanced works on cost-effective oxide-derived copper catalysts for the generation of C2+ products (hydrocarbons and alcohols) and transition metal-nitrogen-doped carbon electrocatalytic materials for C1 compounds production from CO2RR. We think they represent suitable electrocatalyst candidates for scaling up electrochemical CO2 conversion. This short review may provide inspiration for the future design and development of innovative active, cost-effective, selective and stable electrocatalysts with improved properties for either the production of C2+ (alcohols, hydrocarbons) or carbon monoxide from CO2RR.C.M. S.–S. thanks the funding of Sorbonne Université - China Scholarship Council program 2017 and Labex Matisse program (ASDB/2017-12) for the PhD contract of L. Zhang, as well as the ECOS Sud-Chile CONICYT program (Project C17E10). Thanks for the help of Dr. F. J. Recio Cortes and Dr. R. Venegas in Pontificia Universidad Católica de Chile. I.M.-G. would like to thank his postdoctoral contract in the frame of Research Project PTDC/EQU-EPQ/29579/2017, financed by ‘Programa Operacional Regional de Lisboa, na componente FEDER’ and ‘Fundação para a Ciência e Tecnologia, I.P’. J.A. gratefully acknowledge the Spanish Ministry of Economy and Competitiveness (MINECO) under Ramón y Cajal program (RYC-2015-17080).ElsevierUniversidad de Cantabria20202020-10-01journal articlehttp://purl.org/coar/resource_type/c_6501NAhttp://purl.org/coar/version/c_be7fb7dd8ff6fe43info:eu-repo/semantics/articlehttp://hdl.handle.net/10902/20736Current Opinion in Electrochemistry, 2020, 23, 65-73reponame:UCrea Repositorio Abierto de la Universidad de Cantabriainstname:Universidad de Cantabria (UC)Inglésengopen accesshttp://purl.org/coar/access_right/c_abf2Attribution-NonCommercial-NoDerivatives 4.0 Internationalhttp://creativecommons.org/licenses/by-nc-nd/4.0/info:eu-repo/semantics/openAccessoai:repositorio.unican.es:10902/207362026-06-02T12:39:31Z |
| dc.title.none.fl_str_mv |
Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts Electrochemical CO2 reduction reaction on copper oxides and metal-nitrogen- carbon catalysts for value-added products generation |
| title |
Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts |
| spellingShingle |
Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts Zhang, Lin Carbon dioxide electrochemical reduction reaction Electrocatalysis Oxide-derived copper catalysts Transition metal–nitrogen–carbon catalysts Value-added products |
| title_short |
Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts |
| title_full |
Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts |
| title_fullStr |
Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts |
| title_full_unstemmed |
Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts |
| title_sort |
Electrochemical CO2 reduction reaction on cost-effective oxide-derived copper and transition metal-nitrogen-carbon catalysts |
| dc.creator.none.fl_str_mv |
Zhang, Lin Merino García, Iván Albo Sánchez, Jonathan|||0000-0001-6781-5704 Sánchez Sánchez, Carlos Manuel |
| author |
Zhang, Lin |
| author_facet |
Zhang, Lin Merino García, Iván Albo Sánchez, Jonathan|||0000-0001-6781-5704 Sánchez Sánchez, Carlos Manuel |
| author_role |
author |
| author2 |
Merino García, Iván Albo Sánchez, Jonathan|||0000-0001-6781-5704 Sánchez Sánchez, Carlos Manuel |
| author2_role |
author author author |
| dc.contributor.none.fl_str_mv |
Universidad de Cantabria |
| dc.subject.none.fl_str_mv |
Carbon dioxide electrochemical reduction reaction Electrocatalysis Oxide-derived copper catalysts Transition metal–nitrogen–carbon catalysts Value-added products |
| topic |
Carbon dioxide electrochemical reduction reaction Electrocatalysis Oxide-derived copper catalysts Transition metal–nitrogen–carbon catalysts Value-added products |
| description |
The electrochemical CO2 reduction reaction (CO2RR) either to generate multicarbon (C2+) or single carbon (C1) value-added products provides an effective and promising approach to mitigate the high CO2 concentration in the atmosphere and promote energy storage. However, cost-effectiveness of catalytic materials limits practical application of this technology in the short term. Herein, we summarize and discuss recent and advanced works on cost-effective oxide-derived copper catalysts for the generation of C2+ products (hydrocarbons and alcohols) and transition metal-nitrogen-doped carbon electrocatalytic materials for C1 compounds production from CO2RR. We think they represent suitable electrocatalyst candidates for scaling up electrochemical CO2 conversion. This short review may provide inspiration for the future design and development of innovative active, cost-effective, selective and stable electrocatalysts with improved properties for either the production of C2+ (alcohols, hydrocarbons) or carbon monoxide from CO2RR. |
| publishDate |
2020 |
| dc.date.none.fl_str_mv |
2020 2020-10-01 |
| dc.type.none.fl_str_mv |
journal article http://purl.org/coar/resource_type/c_6501 NA http://purl.org/coar/version/c_be7fb7dd8ff6fe43 |
| dc.type.openaire.fl_str_mv |
info:eu-repo/semantics/article |
| format |
article |
| dc.identifier.none.fl_str_mv |
http://hdl.handle.net/10902/20736 |
| url |
http://hdl.handle.net/10902/20736 |
| dc.language.none.fl_str_mv |
Inglés eng |
| language_invalid_str_mv |
Inglés |
| language |
eng |
| dc.rights.none.fl_str_mv |
open access http://purl.org/coar/access_right/c_abf2 Attribution-NonCommercial-NoDerivatives 4.0 International http://creativecommons.org/licenses/by-nc-nd/4.0/ |
| dc.rights.openaire.fl_str_mv |
info:eu-repo/semantics/openAccess |
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open access http://purl.org/coar/access_right/c_abf2 Attribution-NonCommercial-NoDerivatives 4.0 International http://creativecommons.org/licenses/by-nc-nd/4.0/ |
| eu_rights_str_mv |
openAccess |
| dc.publisher.none.fl_str_mv |
Elsevier |
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Elsevier |
| dc.source.none.fl_str_mv |
Current Opinion in Electrochemistry, 2020, 23, 65-73 reponame:UCrea Repositorio Abierto de la Universidad de Cantabria instname:Universidad de Cantabria (UC) |
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Universidad de Cantabria (UC) |
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UCrea Repositorio Abierto de la Universidad de Cantabria |
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UCrea Repositorio Abierto de la Universidad de Cantabria |
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1869407086873411584 |
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15.301603 |