The right computational recipe for olefin metathesis with ru-based catalysts: the whole mechanism of ring-closing olefin metathesis

The initiation mechanism of ruthenium methylidene complexes was studied detailing mechanistic insights of all involved reaction steps within a classical olefin metathesis pathway. Computational studies reached a good agreement with the rarely available experimental data and even enabled to complemen...

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Detalles Bibliográficos
Autores: Poater Teixidor, Albert, Pump, Eva, Vummaleti, Sai Vikrama Chaitanya, Cavallo, Luigi
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2014
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:10256/10349
Acceso en línea:http://hdl.handle.net/10256/10349
Access Level:acceso embargado
Palabra clave:Metàtesi (Química)
Metathesis (Chemistry)
Ruteni
Ruthenium
Mecanismes de reacció (Química)
Reaction mechanisms (Chemistry)
Descripción
Sumario:The initiation mechanism of ruthenium methylidene complexes was studied detailing mechanistic insights of all involved reaction steps within a classical olefin metathesis pathway. Computational studies reached a good agreement with the rarely available experimental data and even enabled to complement them. As a result, a highly accurate computational and rather cheap recipe is presented