Capturing electronic substituent effect with effective atomic orbitals

The occupations of the effective atomic orbitals (eff-AOs) of the carbon atoms in the aromatic ring serve as the basis for deriving accurate descriptors of the inductive (F) and resonance (R) effects exerted by substituents in substituted benzene derivatives. The eff-AOs enable a clear separation of...

Descripción completa

Detalles Bibliográficos
Autores: Comas Vilà, Gerard, Salvador Sedano, Pedro
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2025
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:10256/27294
Acceso en línea:http://hdl.handle.net/10256/27294
Access Level:acceso abierto
Palabra clave:Orbitals moleculars
Molecular orbitals
Descripción
Sumario:The occupations of the effective atomic orbitals (eff-AOs) of the carbon atoms in the aromatic ring serve as the basis for deriving accurate descriptors of the inductive (F) and resonance (R) effects exerted by substituents in substituted benzene derivatives. The eff-AOs enable a clear separation of the σ-type electron density into contributions originating from the C–H/X bonds (where X represents a substituent) and those from the C–C bonding framework. Our analysis reveals that the inductive effect of a substituent is effectively captured by the shift in the occupation of the eff-AOs associated with the C–C bonding framework at the meta position. In contrast, the resonance effect is well-described by the shifts in the occupations of the 2pz-type eff-AOs at the ortho and para positions. The two introduced descriptors for inductive and resonant effects, namely IX and RX, are also applied to predict Hammett's σm and σp in meta- and para-substituted benzoic acid derivatives. In the case of the meta-substituted derivatives, the predictions of the σm values are excellent, with a mean average error of just 0.04. This approach provides a robust and systematic framework for quantifying substituent effects in aromatic systems