Magnetic properties of spinel-type oxides NiMn2-xMexO4

New materials, based on the well-known spinel compound NiMn2O4, have been synthesized and characterized from the magnetic point of view. The manganese cation was partially substituted in the general formula NiMn2-xMexO4 , by nonmagnetic and magnetic elements, such as Me = Ga, Zn, Ni and Cr (0 x 1)....

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Detalles Bibliográficos
Autores: Gautier, J.L., Moure Jiménez, Carlos, Bodenez, V., Cailleaux, X., Ortiz, Juan, Peña, Octavio, Piriou, B., Zúñiga, G., Lisboa-Filho, P. N.
Tipo de recurso: artículo
Fecha de publicación:2005
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/2180
Acceso en línea:http://hdl.handle.net/10261/2180
Access Level:acceso abierto
Palabra clave:Magnetic oxides
Spinels
Ferrimagnetic properties
Magnetic exchange
Descripción
Sumario:New materials, based on the well-known spinel compound NiMn2O4, have been synthesized and characterized from the magnetic point of view. The manganese cation was partially substituted in the general formula NiMn2-xMexO4 , by nonmagnetic and magnetic elements, such as Me = Ga, Zn, Ni and Cr (0 x 1). Prior to the determination of their magnetic properties, the non-substituted spinel NiMn2O4 was carefully characterized and studied as a function of the oxygen stoichiometry, based on the influence of the annealing atmosphere and quenching rate. The ferrimagnetic character was observed in all samples, with a paramagnetic-to-ferromagnetic transition temperature Tc stabilized at 110 K, and well defined long-range antiferromagnetic interactions at lower temperatures, which depend on the applied field and the substitute concentration