Evaluation of matrix effects in the analysis of volatile organic compounds in whole blood with solid phase microextraction

The complexity and matrix variability of biological samples requires an accurate evaluation of matrix effects. Dilution of the biological sample is the simplest way to reduce or avoid the matrix effect. In the present study, a set of volatile organic compounds with different volatilities was used to...

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Detalles Bibliográficos
Autores: Alonso Roura, Mònica, Castellanos Rodrigo, Mar, Sánchez Navarro, Juan Manuel
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2013
País:España
Institución:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:10256/19559
Acceso en línea:http://hdl.handle.net/10256/19559
Access Level:acceso abierto
Palabra clave:Síntesi en fase sólida
Compostos orgànics volàtils
Sang -- Anàlisi
Solid-phase synthesis
Volatile organic compounds
Blood -- Analysis
Descripción
Sumario:The complexity and matrix variability of biological samples requires an accurate evaluation of matrix effects. Dilution of the biological sample is the simplest way to reduce or avoid the matrix effect. In the present study, a set of volatile organic compounds with different volatilities was used to assess the effect of the dilution of blood samples on the extraction efficiency by headspace solid phase microextration. It was found that there was a significant matrix effect, but that this effect differs significantly depending on the volatility of the compound. A 1:2 (blood:water) dilution was enough to allow quantitative recoveries of those compounds VOCs with boiling points <100ºC. For compounds with boiling points between 100-150ºC, the matrix effect was stronger and a 1:5 dilution was required. The dilution of blood samples proved to be inefficient for quantitative recovery of compounds with boiling points >150ºC. A 1:5 dilution of the sample allowed detection limits in the range of of ng/L to be obtained. This was sufficient to detect the main volatile compounds present in blood and contamination after exposure