Practical solvent-free microwave-assisted hydroboration of alkynes

A simple and rapid protocol for the anti-Markovnikov hydroboration of alkynes assisted by microwave irradiation has been developed. Pinacolborane smoothly reacts with terminal alkynes to obtain (E)-alkenyl boronates in good yields and short reactions times in the absence of solvent. Further transfor...

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Detalles Bibliográficos
Autores: Altarejos Salido, Julia|||0000-0002-2871-8597, Sucunza Sáenz, David|||0000-0002-3307-4204, Vaquero López, Juan José|||0000-0002-3820-9673, Carreras Pérez Aradros, Javier|||0000-0002-1521-6758
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universidad de Alcalá (UAH)
Repositorio:e_Buah Biblioteca Digital Universidad de Alcalá
Idioma:inglés
OAI Identifier:oai:ebuah.uah.es:10017/43407
Acceso en línea:http://hdl.handle.net/10017/43407
https://dx.doi.org/10.1002/ejoc.202000110
Access Level:acceso abierto
Palabra clave:Alkynes
Hydroboration
Microwave chemistry
Alkenyl boronates
Solvent-free synthesis
Química
Chemistry
Descripción
Sumario:A simple and rapid protocol for the anti-Markovnikov hydroboration of alkynes assisted by microwave irradiation has been developed. Pinacolborane smoothly reacts with terminal alkynes to obtain (E)-alkenyl boronates in good yields and short reactions times in the absence of solvent. Further transformations on the carbon-boron bond of the adducts can be sequentially achieved without the need of purifying the alkenyl boronates.