Fourier transform infrared spectroscopy of twisted bilayer graphene
(English) The goal of this thesis is to probe the infrared optical response of twisted bilayer graphene (TBG) using Fourier transform infrared spectroscopy (FTIR). First, I used a commercial FTIR to measure the TBG in the mid-infrared range at room temperature. I improved the device fabrication tech...
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| Formato: | tesis doctoral |
| Fecha de publicación: | 2025 |
| País: | España |
| Recursos: | Universitat Politècnica de Catalunya (UPC) |
| Repositorio: | UPCommons. Portal del coneixement obert de la UPC |
| Idioma: | inglés |
| OAI Identifier: | oai:upcommons.upc.edu:2117/428051 |
| Acesso em linha: | https://hdl.handle.net/2117/428051 https://dx.doi.org/10.5821/dissertation-2117-428051 |
| Access Level: | acceso abierto |
| Palavra-chave: | Fourier Transform Infrared Spectroscopy Twisted Bilayer Graphene 535 - Òptica 543 - Química analítica Àrees temàtiques de la UPC::Física Àrees temàtiques de la UPC::Enginyeria química |
| Resumo: | (English) The goal of this thesis is to probe the infrared optical response of twisted bilayer graphene (TBG) using Fourier transform infrared spectroscopy (FTIR). First, I used a commercial FTIR to measure the TBG in the mid-infrared range at room temperature. I improved the device fabrication technique and fabricated the TBG devices with a large area and simultaneously a low inhomogeneity. I observe that the TBG has abundant optical absorption features originating from the interband transitions that are uniquely determined by the twist angle. Then, I want to probe the interband transition of the TBG that lies in the terahertz range, which evolves the flat band of the TBG that hosts strongly correlated effects. I built a homemade FTIR that works in both the mid-infrared and terahertz range. I wired the cryostat carefully and achieved an electrical noise level approaching the Johnson noise limit. By guiding the light from the FITR into the cryostat, I successfully measured the exciton states in the Bernal bilayer graphene device over a broad spectral range, demonstrating that the system is ready for future experimental study of TBG. |
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