Electronic structure of the 2D electron Gasat the AlO_x/KTaO_3(110) interface

Oxide-based 2D electron gases (2DEGs) have generated significant interest due to their potential for discovering novel physical properties. Among these, 2DEGs formed in KTaO3 stand out due to the recently discovered cristal face-dependent superconductivity and large Rashba splitting, both of which h...

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Detalles Bibliográficos
Autores: Martínez, Emanuel Alberto, Dai, Ji, Tallarida, Massimo, Nemes, Norbert Marcel, Bruno, Flavio Yair
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/110421
Acceso en línea:https://hdl.handle.net/20.500.14352/110421
Access Level:acceso abierto
Palabra clave:538.9
2DEG
ARPES
Electronic structure
KTaO3
Rashba spin-orbit coupling
Surface
Superconductivity
Conduction
Systems
Liquid
Física de materiales
2211 Física del Estado Sólido
Descripción
Sumario:Oxide-based 2D electron gases (2DEGs) have generated significant interest due to their potential for discovering novel physical properties. Among these, 2DEGs formed in KTaO3 stand out due to the recently discovered cristal face-dependent superconductivity and large Rashba splitting, both of which hold potential for future oxide electronics devices. In this work, angle-resolved photoemission spectroscopy is used to study the electronic structure of the 2DEG formed at the (110) surface of KTaO_3 after deposition of a thin Al layer. The experiments reveal a remarkable anisotropy in the orbital character of the electron-like dispersive bands, which form a Fermi surface consisting of two elliptical contours with their major axes perpendicular to each other. The measured electronic structure is used to constrain the modeling parameters of self-consistent tight-binding slab calculations of the band structure. In these calculations, an anisotropic Rashba splitting is found with a value as large as 4 meV at the Fermi level along the [−110] crystallographic direction. This large unconventional and anisotropic Rashba splitting is rationalized based on the orbital angular momentum formulation. These findings provide insights into the interpretation of spin-orbitronics experiments and help to constrain models for superconductivity in the KTO(110)-2DEG system.