Microhardness and wear behavior of nanodiamond-reinforced nanocomposites for dental applications

In polymer-based dental composites, wear is a three-body wear system mainly abrasive, because of the food particles and wear products suspended in the oral cavity, which are transferred to the microcavities of the surface of the replacements. Due to this fact, the incorporation of nanodiamond as rei...

Descripción completa

Detalles Bibliográficos
Autores: Moriche Tirado, Rocío, Chetwani, Bhanu, Artigas-Arnaudas, Joaquín, Sánchez, María, Campo, Mónica, Prolongo, Margarita G., Rams, Joaquín, Prolongo, Silvia G., Ureña, Alejandro
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2024
País:España
Institución:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/165720
Acceso en línea:https://hdl.handle.net/11441/165720
https://doi.org/10.1002/pc.29104
Access Level:acceso abierto
Palabra clave:Hardness
Nanodiamond
Photocuring
Polymer–matrix composite
Wear
Descripción
Sumario:In polymer-based dental composites, wear is a three-body wear system mainly abrasive, because of the food particles and wear products suspended in the oral cavity, which are transferred to the microcavities of the surface of the replacements. Due to this fact, the incorporation of nanodiamond as reinforcement in these polymer–matrix composites, which promotes the creation of a solid lubricant tribofilm surface could be advantageous. With the reinforcement of nanodiamonds, BisGMA/TEGDMA-based composites increase their microhardness by 95%–420%. A maximum hardness exceeding 65 HV is achieved with a reinforcement of 3.2 wt%. The specific wear rate of neat BisGMA/TEGDMA is near 10−4 mm3/Nm and the Archard's coefficient is 2.6 × 105. The incorporation of a content of 1.6 wt% ND is enough to cause a diminution of ~78% in the friction coefficient and a reduction of the specific wear rate and Archard's coefficient of ~50%. Nevertheless, the addition of relatively high contents reduces the effectiveness of photoinitiation and photocuring, which is related to the scattering and absorption of light radiation by ND. This causes a significant decline in elastic properties starting at 50 μm from the surface.