A Preliminary Comparative Study of the Baylis–Hillman Reaction in Ionic Liquid Solution and Gelled Ionic Liquid

Baylis–Hillman reaction in ionic liquid ([BMIM][PF]) solution under stirring conditions and in the presence of a base (DABCO) can also be performed efficiently in non-stirred gel phase upon gelation of the ionic liquid using a LMW gelator (i.e., (S)-N-(1-oxo-3-phenyl-1-(tridecylamino)propan-2-yl)ben...

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Detalles Bibliográficos
Autores: Schön, Eva-María, Saldías, César, Haldar, Debasish, Díaz Díaz, David
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2019
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/188299
Acceso en línea:http://hdl.handle.net/10261/188299
Access Level:acceso abierto
Palabra clave:Ionogel
Supramolecular gel
Ionic liquid
Baylis–Hillman reaction
Descripción
Sumario:Baylis–Hillman reaction in ionic liquid ([BMIM][PF]) solution under stirring conditions and in the presence of a base (DABCO) can also be performed efficiently in non-stirred gel phase upon gelation of the ionic liquid using a LMW gelator (i.e., (S)-N-(1-oxo-3-phenyl-1-(tridecylamino)propan-2-yl)benzamide). In this preliminary study, the authors have compared both reaction media and the results showed similar behaviors. Interestingly, the ionogel is found to be slightly more effective affording the desired products with moderately higher yields within a reaction period of 24 h.