On the existence of organometallic palladium(IV) complexes

The reactions of palladium(II) compounds of the type Cl2PdL2 with bromobis(pentafluorophenyl)thallium(III) has been reexamined. The reported preparation of the organo palladium(IV) complex Cl2Pd(C6F5)2(PPh3)2 could not be repeated, and instead mixtures of binuclear palladium(II) compounds, Cl2Pd(C6F...

Descripción completa

Detalles Bibliográficos
Autores: Usón Lacal, R., Royo Gracia, Pascual, Forniés, J., Martínez, F.
Tipo de recurso: artículo
Fecha de publicación:1975
País:España
Institución:Universidad de Alcalá (UAH)
Repositorio:e_Buah Biblioteca Digital Universidad de Alcalá
Idioma:inglés
OAI Identifier:oai:ebuah.uah.es:10017/4937
Acceso en línea:http://hdl.handle.net/10017/4937
https://dx.doi.org/10.1016/S0022-328X(00)88130-9
Access Level:acceso abierto
Palabra clave:Organometallic palladium(IV) complexes
Ciencia
Química inorgánica
Science
Chemistry, inorganic
Descripción
Sumario:The reactions of palladium(II) compounds of the type Cl2PdL2 with bromobis(pentafluorophenyl)thallium(III) has been reexamined. The reported preparation of the organo palladium(IV) complex Cl2Pd(C6F5)2(PPh3)2 could not be repeated, and instead mixtures of binuclear palladium(II) compounds, Cl2Pd(C6F5)2L2, and mononuclear palladium(II) compounds were obtained. The binuclear are transformed into the mononuclear complexes on addition of an excess of ligand L. The chlorine bridging atoms of the binuclear complexes can be replaced by other halogens or pseudohalogens by treatment with salts of the MX type (X = Br, I, SCN).