Poly(epsilon-caprolactone)/Graphene oxide composite systems: a comparative study on hydrolytic degradation at extreme pH values

[EN] Polycaprolactone/Graphene oxide (PCL/GO) composites are shown to be promising substrates for tissue engineering as their degradation behavior is a key aspect in this type of application. The present paper studies the effect of different GO contents (0.1, 0.2 and 0.5 wt%) of PCL/GO composites on...

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Detalles Bibliográficos
Autores: Campillo-Fernández, Alberto J.|||0000-0002-2978-5994, Vidaurre, Ana|||0000-0003-3394-1176, González-Reed, Pablo, Castilla Cortázar, María Isabel Cecilia
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/171694
Acceso en línea:https://riunet.upv.es/handle/10251/171694
Access Level:acceso abierto
Palabra clave:Polycaprolactone
Graphene oxide
Nanocomposite
Hydrolytic degradation
Accelerated degradation
MAQUINAS Y MOTORES TERMICOS
FISICA APLICADA
Descripción
Sumario:[EN] Polycaprolactone/Graphene oxide (PCL/GO) composites are shown to be promising substrates for tissue engineering as their degradation behavior is a key aspect in this type of application. The present paper studies the effect of different GO contents (0.1, 0.2 and 0.5 wt%) of PCL/GO composites on accelerated hydrolytic degradation at pH 13 and pH 1. Degradation kinetics at pH 13 is strongly affected by GO content, and speed up at higher percentages. The composite with 0.5 wt% of GO was completely degraded in 72 hours, while degradation at pH 1 presents a different profile and seems to have an induction period that lasts more than 1500 hours. Morphological changes, molecular weight distribution, weight loss, degree of swelling and calorimetric properties were obtained as a function of degradation time. According to the results obtained, the addition of small percentages of GO significantly influences the degradation behavior of the composites acting as degradation modulators.