Optically active Er3+ ions in SiO2 codoped with Si nanoclusters

Optical properties of directly excited erbium (Er3+) ions have been studied in silicon rich silicon oxide materials codoped with Er3+. The spectral dependence of the direct excitation cross section (σdir) of the Er3+ atomic I415/2→I411/2 transition (around 0.98 μm) has been measured by time resolved...

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Detalles Bibliográficos
Autores: Navarro Urrios, Daniel, Lebour, Youcef, Jambois, Olivier, Garrido Fernández, Blas, Pitanti, Alessandro, Daldosso, Nicola, Pavesi, Lorenzo, Cardin, J., Hijazi, K., Khomenkova, L., Gourbilleau, Fabrice, Rizk, Richard
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2009
País:España
Institución:Universidad de Barcelona
Repositorio:Dipòsit Digital de la UB
OAI Identifier:oai:diposit.ub.edu:2445/15662
Acceso en línea:https://hdl.handle.net/2445/15662
Access Level:acceso abierto
Palabra clave:Matèria condensada
Espectroscòpia
Cristal·lografia
Condensed matter
Spectroscopy
Crystallography
Descripción
Sumario:Optical properties of directly excited erbium (Er3+) ions have been studied in silicon rich silicon oxide materials codoped with Er3+. The spectral dependence of the direct excitation cross section (σdir) of the Er3+ atomic I415/2→I411/2 transition (around 0.98 μm) has been measured by time resolved μ-photoluminescence measurements. We have determined that σdir is 9.0±1.5×10−21 cm2 at 983 nm, at least twice larger than the value determined on a stoichiometric SiO2 matrix. This result, in combination with a measurement of the population of excited Er3+ as a function of the pumping flux, has allowed quantifying accurately the amount of optically active Er3+. This concentration is, in the best of the cases, 26% of the total Er population measured by secondary ion mass spectrometry, which means that only this percentage could provide optical gain in an eventual optical amplifier based on this material.