Iron-Based Core-Shell Nanowires for Combinatorial Drug Delivery and Photothermal and Magnetic Therapy

Combining different therapies into a single nanomaterial platform is a promising approach for achieving more efficient, less invasive, and personalized treatments. Here, we report on the development of such a platform by utilizing nanowires with an iron core and iron oxide shell as drug carriers and...

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Detalles Bibliográficos
Autores: Martínez-Banderas, Aldo Isaac, Aires, Antonio, Quintanilla, Marta, Holguin Lerma, Jorge Alberto, Lozano-Pedraza, Claudia, Teran, Francisco José, Moreno Garcia, Julian, Perez, Jose E., Ooi, Boon S., Ravasi, Timothy, Merzaban, Jasmeen S., Cortajarena, Aitziber L., Kosel, Jürgen
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2019
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/240727
Acceso en línea:http://hdl.handle.net/10261/240727
Access Level:acceso abierto
Palabra clave:Iron−iron oxide core−shell
Nanowires
Photothermal therapy
Magnetic cancer therapy
Drug delivery
Descripción
Sumario:Combining different therapies into a single nanomaterial platform is a promising approach for achieving more efficient, less invasive, and personalized treatments. Here, we report on the development of such a platform by utilizing nanowires with an iron core and iron oxide shell as drug carriers and exploiting their optical and magnetic properties. The iron core has a large magnetization, which provides the foundation for low-power magnetic manipulation and magnetomechanical treatment. The iron oxide shell enables functionalization with doxorubicin through a pH-sensitive linker, providing selective intracellular drug delivery. Combined, the core–shell nanostructure features an enhanced light–matter interaction in the near-infrared region, resulting in a high photothermal conversion efficiency of >80% for effective photothermal treatment. Applied to cancer cells, the collective effect of the three modalities results in an extremely efficient treatment with nearly complete cell death (∼90%). In combination with the possibility of guidance and detection, this platform provides powerful tools for the development of advanced treatments.