Correction of the Shape Effect on Magnetic Entropy Change in Ball Milled Fe70Zr30 Alloys

The field dependence of the magnetic entropy change (ΔSM) after mechanical alloying of Fe70Zr30 composition starting from high purity powders is studied. Samples with different shapes and different crystalline fraction X were analyzed. Although the results show that the proposed correction of the de...

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Detalles Bibliográficos
Autores: Manchón Gordón, Alejandro F., Ipus Bados, Jhon Jairo, Moreno Ramírez, Luis Miguel, Blázquez Gámez, Javier Sebastián, Conde Amiano, Clara Francisca, Franco García, Victorino, Conde Amiano, Alejandro
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2018
País:España
Institución:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/147216
Acceso en línea:https://hdl.handle.net/11441/147216
https://doi.org/10.1016/j.jallcom.2018.06.176
Access Level:acceso abierto
Palabra clave:Amorphous alloys
Magnetocaloric effect
Mechanical alloying
Descripción
Sumario:The field dependence of the magnetic entropy change (ΔSM) after mechanical alloying of Fe70Zr30 composition starting from high purity powders is studied. Samples with different shapes and different crystalline fraction X were analyzed. Although the results show that the proposed correction of the demagnetizing field has not a significant effect on ΔSM(T) curves (∼5% underestimation), it is necessary in order to properly analyze the field dependence of this magnitude (|ΔSM|=aHn). This correction allows recovering the theoretically predicted field dependence as well as a deeper analysis on multiphase systems. In fact, the biphasic character of the studied system changes the value of the field exponent n: it decreases below two above Curie temperature (TC), and it increases at TC. We show that, assuming a non-interacting phase model, it is possible to obtain the value of the exponent n for the main phase from the intercept of n vs X/ΔSM.