Lithogenic and anthropogenic origin of trace elements in surface soils from Amynteo-Ptolemais-Kozani lignite basin

The concentrations of 45 trace elements were determined by ICP-MS in twelve uncultivated surface soil samples inside (S1, S2, S4-S10) and outside (S3, S11, S12) the Amynteo-Ptolemais-Kozani lignite basin, in six surrounding rock samples as well as in a composite fly ash sample. The six rock samples...

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Detalles Bibliográficos
Autores: Georgakopoulos, Andreas, Filippidis, A., Fernandez-Turiel, J. L., Kassoli-Fournaraki, Anna, Iordanidis, A.
Tipo de recurso: otro
Fecha de publicación:2002
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/209298
Acceso en línea:http://hdl.handle.net/10261/209298
Access Level:acceso abierto
Palabra clave:trace elements
Soils
geochemistry
Amynteo
Ptolemais
Kozani
Grecia
Greece
Descripción
Sumario:The concentrations of 45 trace elements were determined by ICP-MS in twelve uncultivated surface soil samples inside (S1, S2, S4-S10) and outside (S3, S11, S12) the Amynteo-Ptolemais-Kozani lignite basin, in six surrounding rock samples as well as in a composite fly ash sample. The six rock samples were chosen to be representative of the surrounding formations of the lignite basin, gneisses, limestones, ophiolites and granites. Equal quantities of fly ash from the four main Power Stations (Agios Dimitrios, Kardia, Ptolemais, Amynteo) were carefully mixed and homogenized to obtain the composite fly ash sample. The enrichment factors, which are the ratio of an element concentration to that of the worldwide average for surface soils, are also determined for all analyzed samples. The concentrations of the elements As, B, Ba, Be, Bi, Cd, Ce, Cs, Cu, Dy, Er, Eu, Ga, Gd, Hf, Hg, Ho, La, Li, Mo, Nb, Nd, Pb, Pr, Rb, Sb, Sc, Sm, Sn, Sr, Ta, Tb, Th, U, V, Y and Zr, are more or less similar to the worldwide surface soils average, with enrichment factors <3.0. Three elements (Ag, Ge and Se) showed enrichment factors >3.0 in all soil samples, Ni in ten soil samples, Cr in seven, Zn in three, Co in two and Win one soil sample. The enrichment of the elements Co and W is mainly attributed to lithogenic (surrounding rocks) influences, while the enrichment of Ge and Se mainly implies anthropogenic influences (intensive lignite exploitation, combustion in Power Stations, fly ash, landfill in external deposits). Both lithogenic and anthropogenic influences are inferred from the enrichment of Ag, Ni, Cr and Zn.