The role of carbon nanotubes in both physical and chemical liquid-solid transition of polydimethylsiloxane

In this work we investigate the effect of the dispersion degree of as-received multiwall carbon nanotubes (MWNTs) in the liquid-solid transitions (LST) of polydimethylsiloxane (PDMS). The physical LST of the suspensions showed a strong dependence on the nanotubes dispersion degree due to the formati...

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Detalles Bibliográficos
Autores: Romasanta, Laura J., López-Manchado, Miguel A., Verdejo, Raquel
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2013
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/194110
Acceso en línea:http://hdl.handle.net/10261/194110
Access Level:acceso abierto
Palabra clave:Carbon nanotubes
Polydimethylsiloxane
Cross-linking reaction
Rheological properties
Dispersion
Descripción
Sumario:In this work we investigate the effect of the dispersion degree of as-received multiwall carbon nanotubes (MWNTs) in the liquid-solid transitions (LST) of polydimethylsiloxane (PDMS). The physical LST of the suspensions showed a strong dependence on the nanotubes dispersion degree due to the formation of an interconnected network as the dispersion time increased. These MWNTs acting as >effective physical cross-links> also influenced the dynamic viscoelastic properties, accelerating the chemical LST (or chemical cross-linking) and giving rise to an increase in the cross-linking density of the composite samples.