Structural and Chemical Evolution of an Inverse CeOx/Cu Catalyst under CO2 Hydrogenation: Tunning Oxide Morphology to Improve Activity and Selectivity

Small nanoparticles of ceria deposited on a powder of CuO display a very high selectivity for the production of methanol via CO2 hydrogenation. CeO2/CuO catalysts with ceria loadings of 5%, 20%, and 50% were investigated. Among these, the system with 5% CeOx showed the best catalytic performance at...

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Detalles Bibliográficos
Autores: Moncada, J., Chen, X., Deng, K., Wang, Y., Xu, W., Marinkovic, N., Zhou, G., Martínez Arias, Arturo, Rodriguez, J.A.
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2023
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/358234
Acceso en línea:http://hdl.handle.net/10261/358234
https://www.scopus.com/inward/record.uri?eid=2-s2.0-85178095784&doi=10.1021%2facscatal.3c04222&partnerID=40&md5=8a454533b62c60c79db03e7df7d22b2b
Access Level:acceso abierto
Palabra clave:carbon dioxide
hydrogen
methanol synthesis
hydrogenation reactions
ceria
copper
in situ characterization
microscopy
Descripción
Sumario:Small nanoparticles of ceria deposited on a powder of CuO display a very high selectivity for the production of methanol via CO2 hydrogenation. CeO2/CuO catalysts with ceria loadings of 5%, 20%, and 50% were investigated. Among these, the system with 5% CeOx showed the best catalytic performance at temperatures between 200 and 350 °C. The evolution of this system under reaction conditions was studied using a combination of environmental transmission electron microscopy (E-TEM), in situ X-ray absorption spectroscopy (XAS), and time-resolved X-ray diffraction (TR-XRD). For 5% CeOx/Cu, the in situ studies pointed to a full conversion of CuO into metallic copper, with a complete transformation of Ce4+ into Ce3+. Images from E-TEM showed drastic changes in the morphology of the catalyst when it was exposed to H2, CO2, and CO2/H2 mixtures. Under a CO2/H2 feed, there was a redispersion of the ceria particles that was detected by E-TEM and in situ TR-XRD. These morphological changes were made possible by the inverse oxide/metal configuration and facilitate the binding and selective conversion of CO2 to methanol. © 2023 American Chemical Society.